This study investigates the potential of
36Cl in tracing young groundwater with residence times of up to ~50 years. Groundwater samples were obtained from 16 irrigation wells in paddy fields located within an upland–lowland system in the Yoro River basin, Central Japan.
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This study investigates the potential of
36Cl in tracing young groundwater with residence times of up to ~50 years. Groundwater samples were obtained from 16 irrigation wells in paddy fields located within an upland–lowland system in the Yoro River basin, Central Japan. The
36Cl/Cl ratios were in the range of 17 to 362 × 10
−15. Among the samples with higher Cl
− concentrations (>10 mg/L), two samples showed high nitrate concentrations as well (>30 mg/L). Except for these samples, the distribution of
36Cl in groundwater was essentially consistent with previous tritium concentration data measured in 1982 and 1994, considering the time that has elapsed since these earlier measurements were performed.
36Cl/Cl values were less than 30 × 10
−15 in lowland areas, with higher values in and around upland areas. The results indicate longer residence times in the regional groundwater flow system (>50 years) than those estimated in previous studies, especially in the area west of the Yoro River. The results demonstrate the ability of
36Cl to trace young groundwater flow, particularly because high values of bomb-derived
36Cl/Cl are easily discriminated from pre-bomb water with low
36Cl/Cl values. Because of its very long half-life (3.01 × 10
5 years),
36Cl remains even after tritium is no longer available.
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