1. Introduction
For the pulsed electric field treatment of plant cells, pulses with voltages in the range of several 10 kV and currents in the order of at least several 100 A are required. Thereby, the Marx circuit is one of the common configurations for the pulse generator [
1]. A basic pulse circuit for one stage of a Marx-type solid-state pulse generator for the generation of unipolar pulses comprises a capacitor, a solid-state switch, and a free-wheeling diode. After closing the switch, the capacitor delivers its stored energy into the connected load. The energy transfer ends if either the complete stored energy has been transferred to the load or the switch has been opened. In the case of an inductive component of the impedance of the attached load, the current may commutate to the current path through the free-wheeling diode. If the switch has previously opened, this prevents the occurrence of an over-voltage across the switch.
This basic circuit can be stacked. The charging path can be set up using solid-state switches comprising additional active switches [
2]. When charging the stage capacitors in a parallel configuration, the power supply needs to have the characteristic of a current source in order to provide direct control of the charging current.
The Marx generator features voltage multiplication according to the number of stages and the voltage stress of each component to be limited to the stage voltage only [
3]. Both advantages are achieved by the combination of charging the capacitors in a parallel configuration and discharging them in a series configuration, and, moreover, by adding circuit elements, i.e., inductors or resistors, in between the stages providing a DC current flow during charging and transient insulation during pulse generation. This concept has been varied, in particular with respect to the arrangement of the current path for charging. In [
4,
5], pulse circuits with voltage multiplication and resonant charging are described. Both circuits feature circuit elements, i.e., diodes and transformers, providing the required insulation between stages during pulse generation, which are stressed with a pulse voltage which is significantly higher than the stage voltage. Article [
6] describes a charging circuit featuring a voltage source with a series resistor and some diodes, which bridge several stages and, hence, need to block more than only the stage voltage. In [
7], a pulse transformer is used for distributing the gate signals to the generator’s IGBT switches, which needs to be designed to insulate the peak pulse voltage. According to [
8], a boost converter configuration acting as a current source and delivering a bipolar output voltage delivers current to the charging path, which is equipped with diodes and MOSFET switches designed to block the stage voltage only.
The goal of the investigations described in this paper is to set up a Marx generator with resonant charging and a design with only one actively controlled switch per stage in order to reduce the effort for control circuitry with respect to designs having more active switches per stage. Moreover, this combination allows advantageously for a fine-tuning of the charging voltage using only the single switch per stage in addition to its original use as a pulse switch.
The pulse shape can be determined by means of appropriate control of the pulse switches allowing for the generation of arbitrary voltage shapes. Such an operation requires stage capacitors, which are sufficiently large to keep the voltage droop during pulse generation small and, hence, allow the generation of almost rectangular voltage shapes. If the controlled variation of the pulse shape is not important, the pulse shape can be determined by the passive circuit elements of the pulse circuit. In the case of the classic Marx generator, this would be an RLC circuit.
The pulse circuit of such an electroporation device comprises the Marx generator, the treatment chamber, and the circuit inductance. The Marx generator serves as capacitance. Thereby, the effective capacitance
C is formed by the series configuration of the stage capacitors
Cstage as given in Equation (1) and depends on the number of stages
n.
The treatment chamber comprises an electrode system for the pulsed electric field applied to the processed material. It can be modelled as an ohmic resistance R. The inductance L can either be formed by the stray inductance of the pulse circuit only or augmented by a coil added to the pulse circuit. The resistance of the treatment chamber may vary with the electric conductivity of the processed material, which depends, among other parameters, on the temperature and the filling factor. As a consequence, the pulse shape may vary.
The solution of the differential Equation (2)
for the initial conditions
and
describes the time characteristic of the voltage across the Marx generator’s effective capacitance
C. The voltage across the resistance
R of the treatment chamber,
(Equations (3)–(5)), can be derived according to [
9]. Thereby, three different cases are distinguished depending on the quality factor
Q as given in Equation (6):
Aperiodic case (
Q < 0.5):
Critically damped case (
Q = 0.5):
Damped periodic case (
Q > 0.5):
with
with the voltage across the resistance R of the treatment chamber,
, the pulse current
ip(t) can be calculated according to Equation (7).
For the pulsed electric field treatment of biological material, a pulse shape similar to the aperiodically damped case or the strongly damped periodic case of an RLC circuit is already in use in industrial-scale electroporation devices equipped with Marx generators [
2]. Therefore, for the new generator design, a Marx-type generator with solid-state switches and an RLC pulse circuit serving as a conventional pulse-forming circuit has been chosen. However, the free-wheeling diodes as part of the pulse generator topology prevent the stage capacitors from being charged in reverse polarity in the case of an oscillatory waveform of the pulse. In this case, as soon as the stage capacitors are discharged, the current driven by the circuit inductance commutates into the free-wheeling diodes and from that moment on, the pulse current decays exponentially, governed by the time constant
of the resulting LR circuit.
Figure 1 shows the simulated pulse voltage V
P and pulse current I
P at the output terminal of an 8-stage Marx generator with free-wheeling diodes. After the discharge of the stage capacitors, the pulse current commutates to the free-wheeling diodes (I
D).
For such a design, a conventional charging circuit equipped with charging coils can be used. However, when operating such a pulse generator at a higher pulse repetition rate and as a consequence, the product of pulse length and pulse repetition rate becomes larger, using current-compensated chokes instead of the charging coils is advantageous for enabling fast charging [
2]. Current-compensated chokes feature a low inductivity during charging, as they are operated in differential mode. During pulse generation, their high inductivity under common-mode conditions serves well for transient stage insulation.
The design based on current-compensated chokes in the charging path can be combined with a power supply having the characteristic of a voltage source and an additional inductance between the power supply and the Marx generator to enable resonant charging of the generator [
10].
Figure 2 shows a simplified circuit for basic studies on resonant charging. The voltage source
V0 supplies energy to the circuit. The capacitance C represents the parallel connection of the generator’s stage capacitors. The inductance L forms together with the capacitance C a resonant circuit. The resistance R represents the resistive losses of the circuit. Initially, the capacitance C is uncharged, and there is no current flow through L, i.e., i(0) = 0. So, there is no energy stored in the circuit. Charging ends when the voltage across the capacitance C reaches its peak value.
The solution of the differential Equation (9)
for the initial conditions
and
describes the time characteristic of the voltage across the paralleled stage capacitors
C for the case of a circuit being initially free of energy. Thereby, depending on the value of the quality factor
Q according to Equation (6), three different cases (
Q < 0.5,
Q = 0.5, and
Q > 0.5) might be considered. However, for efficient charging, the losses represented by R need to be low. Therefore, only the oscillatory case with
Q > 0.5 is of interest. The voltage across the stage capacitors is given by
If the resistance
R is assumed to be zero, the voltage
rises up to a peak value of
. Hence, for such a design, during repetitive operation, the charging voltage of the stage capacitors may reach approximately twice that of the supplying voltage source. Thereby, the initial condition
is guaranteed by a complete discharge of the stage capacitors during the previous pulse. If the initial condition for the current through the inductance
L is modified in such a way, that there is already a significant energy
WL stored in
L, which correlates to an initial current
The initial condition for
becomes
The initial current of the charging process,
i(0), rises with an extended on-time of the stage switches. As long as these switches are closed, the stage capacitors are shorted, and the current through the inductance
L rises according to
However, if the value of the resistance
R is negligibly small, the rise of the current
i(
t) can be approximated to be in proportion to the time according to
The opening of the switches defines the beginning of the charging process as described above. Thereby, the charging voltage can be fine-tuned by means of a modulation of the on-time of the stage switches.
An industrial-scale electroporation device can be designed for an operation around one well-defined operating point. If there is no need for a wide variation of the voltage, the rectified voltage across a DC-link capacitor grounded at its negative pole may serve as a cheap voltage source. An additional transformer may provide the required insulation from the grid.
In order to investigate the operation of the resonant charging circuit of a solid-state switched Marx circuit via current-compensated chokes, circuit simulations of an eight-stage Marx circuit have been performed.
2. Materials and Methods
For the circuit simulation of an 8-stage Marx generator, a circuit model for circuit simulation using the software LTspice [
11] has been set up, which is shown in
Figure 3. Based on the circuit topology and component values, LTspice sets up a system of difference equations and solves them numerically for a sequence of adapted time steps considering the appropriate initial conditions. In between the time steps, linear interpolation is applied [
11]. LTspice has also been used for post-processing, i.e., the calculation of data, which has been derived from the original simulation data, such as, e.g., the integration over time or averaging of a curve.
Each stage is represented by its stage capacitor having the capacitance C_ST = 6 µF, and the solid-state switch, which is modelled using a voltage-controlled switch and an anti-parallel diode representing the internal diode co-packed with many IGBT switches. Additionally, each stage features a bypass diode (D1, D5, D9, D13, D17, D21, D25, and D29 in
Figure 3). The load is modelled as a combined resistive and inductive load (R1 + R2, L16 + L17). The charging path comprises the coupled inductor-pairs (L1, L2), (L3, L4) … (L13, L14), each representing one current-compensated choke. The capacitance between both windings is represented by the sum of the adjacent capacitors (C2 + C3) … (C20 + C21). Each winding has an inductance of
LL = 4.7 mH and resistance of
LR = 5 mΩ. With a coupling coefficient of KPLG = 0.999, very well magnetic coupling between both windings has been assumed. The common-mode current component through one current-compensated choke is obtained by calculating the difference of the currents through both windings. The stages are connected to the charging path via diodes (D3, D4), (D7, D8) … (D31, D32). These diodes prevent the stage capacitors from discharging via the charging path after resonant charging.
The voltage source needed for the resonant charging circuit is modelled by the ideal voltage source V1. The voltage source V1 is paralleled with a capacitance C23 serving in a real setup as a DC-link capacitor. However, for the simulation, this capacitor is not required.
The inductance L15 forms, together with the paralleled stage capacitors, the resonant circuit for resonant charging. Just after pulse generation, the stage capacitors are discharged completely. The bypass diodes of each stage prevent the stage capacitors from being charged at the opposite polarity and, hence, prevent the pulse circuit from oscillating. As soon as the voltage of the stage capacitors falls below the voltage of the power supply, the charging current starts to rise and recharges the stage capacitors in a parallel arrangement. Thereby, the voltage across the stage capacitors reaches approximately twice the voltage of the feeding voltage source.
The values of the stage capacitors, the load, the current-compensated chokes, and the inductance L15 have been selected based on a design for a solid-state Marx generator with a stage voltage of 1 kV delivering pulses with an approximate pulse length
th = 10 µs at a pulse repetition rate of up to 500 Hz to the load. Thereby, the pulse length is measured at half amplitude, and the average power of one stage operating at 1 kV and 500 Hz is 1.5 kW [
10,
12,
13].
In order to generate an output voltage, which is symmetric to ground potential, the pulse generator is grounded at its centre. This arrangement is of advantage for a later connection of a pulsed electric field treatment chamber [
14]. The power supply for charging the generator is isolated to ground potential. During the operation of the real circuit, a varistor may limit the voltage versus ground in case of an over-voltage event.
During pulse generation, some amount of magnetic energy is stored in the chokes resulting in a common-mode current. An accumulation of such energy from pulse to pulse and, hence, an increase in the common-mode current may cause the saturation of the magnetic cores resulting in a loss of inductance. If the common-mode current is interrupted suddenly, an induced voltage may result in an over-voltage causing excessive stress on the insulation. In order to dissipate some of the energy accumulated in the current-compensated chokes between two pulses, a damping resistor R
D (R3 in
Figure 3) has been implemented. It has been added to the circuit in such a way that it is not part of the current path during the charging process and, hence does not cause additional losses during charging.
For the simulations, the value of the damping resistor R3 and the on-time of the switches have been varied, and the effects on the circuit have been studied.
4. Discussion
In order to verify the simulation results, an experimental setup has been made. The results obtained in the simulations have been compared to measurements at an 8-stage Marx generator with similar parameters, as shown in the circuit in
Figure 3. Likewise, it features a damping resistor R
D [
10].
Figure 24 shows the charging current and the charging voltage at the charging input terminal of an 8-stage Marx generator. The on-time of the solid-state switches is 22 µs. The measurement results fit very well with the simulation results shown in
Figure 13 with respect to the charging voltage and charging time and as well as the ringing after charging. Simulation and measurements differ slightly with respect to damping. However, an exact fit of the simulations to measurements was not the goal of the investigations.
Figure 25 shows the measured charging voltage after inserting a diode in series to the charging coil L15. It suppresses the ringing as expected. The measured voltage across the damping resistor R
D exhibits a similar shape as the current I
RD in
Figure 20 and
Figure 21 and shows very well the change of the current path of the common-mode current during charging and the finding that damping of the common-mode current occurs mainly after charging of the generator.
For the eight-stage Marx generator, the power dissipation in the damping resistor RD in the order of 50 W is small compared to the average power which the generator delivers to the load. This power is, on average, 12 kW when operating the generator at a charging voltage of 1 kV per stage and 500 Hz pulse repetition rate. However, the total power of the Marx generator and the energy stored in the cores of the current compensated chokes both scales with the number of stages. The energy that is dissipated in the damping resistor RD scales with the number of current-compensated chokes, which is one less than the number of stages. Hence, the ratio of average power dissipated in RD and the total average power of the generator scales with n/(n + 1). For a large number of stages n, the ratio can be approximated as a linear dependency of the number of stages n. Especially for a Marx generator with a larger number of stages, the heat dissipation at the damping resistor needs to be considered. Moreover, with a damping resistor of RD = 20 Ohm, the amplitude of the common-mode current is significantly higher than for the case without a damping resistor. In the presented simulations, the peak value of the common-mode current with RD = 20 Ohm is 3.2 A under steady-state conditions, and without a damping resistor, only 1.8 A. In the latter case, the current through the current-compensated chokes decays to zero right after charging the capacitors. As a consequence, the cores of the current-compensated chokes in the charging path can be designed smaller.
For a design omitting the damping resistor RD, the power supply needs to be designed in such a way that it can cope with a floating potential at its ground-side terminal. This can be accomplished either by static or transient insulation of the power supply versus ground. Static insulation may comprise a transformer as an insulating element. Dynamic insulation may be achieved by adding a second charging coil LRes also to the ground-side current path between the voltage source V1 and the pulse generator and distributing the total inductance equally among both coils. Together with a capacitance between the output terminals of the power supply V1 and ground potential, these inductances form a second-order low-pass filter. Depending on the design, the stray capacitance between the voltage source and ground might be used advantageously for this purpose.
One feature of the presented design is the possibility of energy-efficient soft-switching under almost zero-current conditions both when closing and opening the switches.
Figure 26 shows the voltage and current at the positive and negative output terminal of the 8-stage generator. As the voltage rises within less than 100 ns while the current is still low, the switching losses are kept small enough to allow for air-cooling of the semiconductor switches with natural convection in repetitive operation [
16]. When using the feature of fine-tuning the charging voltage by means of an extended on-time of the switches, the stage switches open under a zero-voltage condition, as the stage capacitors remain uncharged as long as the switches are closed, and the current commutates just after opening the switches to the current path through the stage capacitor. However, when opening the switches before the stage capacitors have been discharged completely, as shown in
Figure 16, the switches are opened under hard-switching conditions involving additional switching losses. Therefore, such an operation should be omitted under normal operating conditions.