1. Introduction
In the process of industrial development, a large amount of industrial organic wastewater being generated every day is harmful to human health and the environment. Currently, the ways for treating industrial wastewater mainly include physical, chemical, and biological methods. However, these methods cannot fulfill the treatment requirements of organic wastewater well [
1,
2]. In recent years, because of its simple structure [
3,
4], outstanding degradation effect, and zero secondary pollution, the hydrodynamic cavitation degradation technology has gradually become a hot spot in the research of organic wastewater treatment [
5,
6]. Hydrodynamic cavitation can be produced by changes in flow and pressure and its generation is usually based on a specific structure. The self-oscillating pulse jets formed by the self-oscillating nozzle [
7,
8] have a strong cavitation effect in this type of structure [
9]. The research on self-oscillating jet nozzles has an important academic and market value.
Currently known parameters that have a greater impact on the cavitation performance of the SOCJN include the inlet diameter, outlet diameter, chamber diameter, chamber length, collision wall convergence angle, and inlet pressure [
10]. The inlet and outlet diameters and chamber length of the nozzle are very important to the cavitation performance. The change to the collision wall convergence angle directly influences the distribution of jet flow field performance, especially the distribution of the pressure field in the nozzle; the low-pressure area is a key factor for the formation and development of cavitation [
11]. The inlet pressure is the input source of the overall jet energy, which directly influences jet power. Moreover, inlet pressure has a great influence on the cavitation ability and erosion effect of jets [
12]. Li et al. [
13] analyzed and deduced the natural frequency of the organ pipe’s resonant chamber in accordance with the principles of transient flow and hydroacoustic, obtained the design mode, and found that the diameter and length of the resonant chamber were key factors affecting the resonance of resonant fluid through experiments, thus summarizing the design mode of the SOCJN on the basis of the organ pipe’s resonant chamber model. Liu et al. [
14] researched the aeration treatment of the chamber structure; analyzed the diameters, positions, and number of different aeration holes; and proposed a solution of using a structure with front and rear chambers distributed symmetrically, which had a high degree of cavitation.
Researching the influence of the structure parameters of the SOCJN on the internal cavitation jet flow field, Qi et al. [
15] applied a series of methods to establish a two-chamber self-oscillating cavitation nozzle for numerical simulation, obtaining the influence law of the incoming flow Reynolds number and the ratio of the front chamber’s length and diameter to the rear chamber on the cavitation jets. Yuan et al. [
16] took the chamber angle, chamber diameter, chamber length, and outlet diameter as design variables; they then took impact peak value and impact pulsation amplitude as target variables and the order of influence of each factor was obtained. Wang et al. [
17] and Makhsuda et al. [
18] studied the flow field characteristics of the Helmholtz self-oscillating cavitation device based on numerical simulation and concluded that when outlet pressure is constant, the cavitation performance can be enhanced by increasing inlet pressure and the structure with the cone collision wall has the most obvious effect.
In this paper, aiming at optimizing the design of the SOCJN, numerical simulation is carried out for inlet pressure and the structural parameters of the nozzle to evaluate the cavitation ability of the jet flow field and the influence weight of each parameter on the nozzle, which provides a reference for the optimized design of the SOCJN for treating industrial wastewater.
3. Results and Discussion
3.1. Main Effect Analysis
Figure 5 shows the main effect of each design parameter of the SOCJN on the response cavitation number and the VOF [
23]. It can be seen from
Figure 5 that the effect of inlet pressure and C
DD2 on the response variables, including the VOF and the average cavitation number, is negligible as the factor level rises. The increase in C
LD would lead to a plummet in the VOF and an upsurge in the average cavitation number.
With the increase in CD21, the VOF falls after rising while the average cavitation number rises after falling, reaching the extreme point at the position of CD21 = 1.50. The increase in the inlet diameter D1 will lead to a fall in the VOF and a rise in the average cavitation number; but, the influence is not as large as that of CLD and CD21 on the response variables.
3.2. Analysis of Interaction Effect
Figure 6 and
Figure 7 show the interaction effect of each design parameter of the SOCJN on the response cavitation number and VOF [
24]. It can be seen from the figures that C
D21, the ratio of the nozzle outlet diameter to the inlet diameter, has a significant interaction with the high and low points of the inlet diameter D
1. In addition, with the rise in C
D21, the average cavitation number at the high point of D
1 gradually increases and the VOF gradually decreases. The average cavitation number at the low point of D
1 rises after falling and the VOF falls after rising. C
LD, the ratio of the chamber length to its diameter, has a significant interaction with D
1.
With the rise in CLD, the average cavitation number at the high point of D1 gradually increases and the VOF gradually decreases. The average cavitation number at the low point of D1 rises after falling, with the inflection point appearing at CLD = 6; but, the VOF keeps on falling. There is a less significant interaction between CDD2, the ratio of chamber diameter to the outlet diameter, and D1.
3.3. Pareto Plot and Correlation Analysis
Figure 8 shows the correlation diagram of the effect of each design parameter of the SOCJN on the response cavitation number and the VOF [
25]. It can be seen from
Figure 8 that the change in the nozzle inlet pressure pin basically has no effect on the average cavitation number and VOF. They are positively correlated with C
LD, with a correlation degree of around 0.6. D
1 is also positively correlated with them; but, the correlation is not as strong as that of C
LD. C
D21 and C
DD2 are also positively correlated; but, the correlation is weaker. The contribution rate of each design parameter of the SOCJN to the cavitation number σ and the VOF is shown in the Pareto diagram, in which the blue bar represents the positive effect and the red represents the negative.
Figure 8 shows the design parameters of the nozzle. The second-order term and interaction term of the design parameters have opposite contribution rates to the cavitation number and VOF, which is inconsistent with the actual situation, indicating that it is infeasible to judge whether cavitation occurs and determine the cavitation degree with the cavitation number. The VOF is more reliable.
It can be seen from the Pareto diagram of the VOF in
Figure 9 that the dimensionless parameters of C
D21, C
LD, and C
DD2 and the inlet diameter D
1 of the nozzle are all negatively correlated with the VOF; the dimensionless parameter C
LD has the largest contribution rate, followed by C
D21 and C
DD2. C
LD is the ratio of the chamber length L to the chamber diameter D of the nozzle; so, the smaller the value, the better the cavitation performance of the nozzle.
3.4. Mathematical Model
According to the optimization model and approximate model, 501 iterative calculations are carried out using the ISIGHT software; all feasible solution sets are shown in
Figure 10. All points in
Figure 10 are feasible solutions for calculations. All of the points in the green circle are combined as the Pareto frontier and the optimal solution can be selected flexibly according to weight values. In this paper, the Pareto point solution is taken as the final result. One set of optimized data is selected for simulation and the simulated VOF distribution cloud map of the model before and after optimization is shown in
Figure 9.
According to the attached table, since the inlet diameter determines the pressure and velocity levels, the cavitation performance weakens with the increase of the outlet diameter, which may be caused by the hindering effect of the nozzle outlet on the jets. Therefore, a suitable outlet diameter is conducive to reducing the energy loss. When the inlet diameter is 4.7, the outlet of the nozzle can better accept the energy provided by its inlet so that the energy loss is reduced and the cavitation performance is better. Hence, the proportioning relationship between the inlet and outlet of the nozzle is also very important. The pulse occurs when the inlet diameter of the SOCJN is 4.2 mm, 4.6 mm, or 4.9 mm and it becomes the most obvious when the diameter is 4.7 mm. Therefore, the parameter ratio of D2/D1 being between 2.2 and 2.67 is an optimal range and the best result happens when D2/D1 = 2.6. This is found by observing the changes in the chamber that show that the larger the chamber diameter, the larger the low-pressure range; the chamber diameter plays a critical role in deciding whether the vortex ring structure in the chamber is conducive to outputting effective kinetic energy and generating cavitation pockets that can change periodically.
The output of the nozzle outlet energy is also affected by the outlet and the chamber diameter. The optimization results demonstrate that the cavitation being performed is optimal when the ratio of chamber length to chamber diameter equals 0.63. The good cavitation performance of the nozzle is related to not only the high-speed jets at its inlet but also the pulse frequency. At a certain frequency, the uneven energy output of the pulsed jets will cause pressure oscillations in the chamber; but, the continuous alternating stress greatly improves the effect of cavitation. The cavitation performance is the best when the ratio of chamber length to chamber diameter is around 6.8 and the inlet pressure is around 4.8 MPa. Under these conditions, the VOF and cavitation number reach 0.6 and 0.5, respectively, proving that cavitation occurred and has an obvious performance.
3.5. Experimental Verification
An aluminum plate sample is placed squarely facing the SOCJN for a continuous 20 min lashing. Then, the pump is turned off to take out the sample. The obtained cavitation effect is shown in
Figure 11. As shown in
Figure 11, the results of the impact test by the nozzle indicate that the No. 3 nozzle has a relatively obvious impact range, with impacting marks that tend to be deeper from the center to the periphery. The No. 1 nozzle is the optimized nozzle and its impacting marks are smaller and shallower than those of the No. 2 and No. 3 nozzles. Although it causes severe erosion in the center area, the No.2 nozzle causes smaller impacting marks on the periphery, which also proves that the structural parameters of the No. 3 nozzle are a better group in the process of simulation. Adjusted on the basis of the optimal parameters, the No. 3 nozzle has a better impact than the No. 1 and No.2 nozzles. Based on the impact test, the SOCJN has an outstanding cavitation performance, with the capability to cause relatively vigorous cavitation. The feasibility of the SOCJN for refractory industrial wastewater treatment has been confirmed from the perspective of cavitation.
4. Conclusions
In this paper, the structure of the SOCJN is optimized by the optimizing Latin method and response surface method. The main conclusions are as follows:
- (1)
The self-oscillating pulsed jet from the SOCJN has the best cavitation performance at the monitoring point when the diameter of the upper nozzle DL = 4.7 mm, the ratio of the upper diameter of the nozzle to the lower one D1/D2 = 2.6, the ratio of the cavity length to the cavity diameter L/D = 0.63, and the convergence angle of collision wall α = 120°, all of which are optimal structural parameters;
- (2)
When the structural parameters of the nozzle remain unchanged, the velocity at the outlet has a linear relationship with the initial working pressure and the cavitation performance increases with the rise in the initial pressure. When the initial pressure is greater than the threshold value, the cavitation performance begins to deteriorate. When the structural parameters of the nozzle are optimal structural parameters, the cavitation performance is the best at the initial pressure of about 4.8 Mpa;
- (3)
The fitting effect of the response surface approximation model is better than other approximate models. It finds that the second-order response surface approximate model is suitable for the SOCJN. There is an error smaller than 8% between the approximate model results and calculated results of the nozzle response, indicating that the former has high accuracy and the analysis results are reliable. The experimental results verify the reliability of this optimized design scheme.
In this paper, taking the vapor volume fraction as the research objective, a variety of design methods are used to optimize the design of the SOCJN. The relationship between the external geometric parameters of the nozzle and the vapor volume fraction is established and the comparison and verification are made with the experimental results, which provide a theoretical basis for the engineering application of the SOCJN.