1. Introduction
In this paper, we address/readdress several fundamental issues related to the quantum vacuum [
1] in the context of atom-field interactions [
2,
3,
4] pertaining to quantum radiative processes.
Vacuum fluctuations of a quantum field, described as quantum noise in the environment, impart a stochastic component in the dynamics of the system, here, the internal degrees of freedom (idf) of an atom/detector, interacting with a quantum field. Quantum dissipation ensues [
5], obeying a quantum fluctuation-dissipation relation (FDR) (Note two sets of FDRs are involved. When we address the vacuum fluctuations vs. radiation reaction, we refer to the FDR of the free environment field (in its initial state). However, when we compare the FDR in linear response theory vs. nonequilibrium dynamics, it is the FDR of the system (in its final equilibrium state)) of the field [
6,
7,
8,
9], on balance with the quantum noise associated with the vacuum fluctuations in the field. Under specific conditions to be expounded later, radiation of a quantum nature is emitted from the atom. This paper highlights the key issues across this spectrum from vacuum fluctuations in a quantum field to stochastic dynamics of the idf of a moving atom to its emitted quantum radiation. We divide these issues into two groups.
Group A is about the relation of vacuum fluctuation and quantum dissipation, which is often misconstrued as radiation reaction of classical radiation theory. (1) It is the dissipation in the quantum dynamics of atomic system’s internal degree of freedom engendered by the vacuum fluctuations of the environmental field. Vacuum fluctuation is intrinsically quantum in nature while radiation reaction exists at the classical level. When referring to this dualism, for conceptual clarity, we suggest replacing the term ‘radiation reaction’ by quantum dissipation, or adding the word ‘quantum’ to it. (2) Vacuum fluctuations are related to quantum dissipation by a fluctuation-dissipation relation. This relation does not connect vacuum fluctuations with classical radiation reaction. Vacuum fluctuations can be viewed (and for Gaussian fields, equated with, by way of the Feynman-Vernon functional identity) as quantum noise. What spanned two decades of debates (from the early 70s to 90s [
10,
11,
12,
13]) mixed with some degree of confusion on this issue stems from the protagonists not recognizing that a distinct level of structure, namely, the stochastic, is organically tied to the quantum. Many introduced noise as an ad hoc entity added in by hand to the classical narrative. To avoid confusion it is important to place each issue under discussion in its appropriate level of theoretical structure. This theme is discussed in
Section 2. Group A issues were already expounded in the work of Johnson and Hu [
5,
14]. We lay out these issues here for the sake of conceptual clarity, leaving much details to these earlier work. Here we wish to highlight the FDR in two aspects: (a) showing the differences between FDRs defined in the context of the nonequilibrium (NEq) dynamics of open quantum systems and FDRs defined conventionally in linear response theory (LRT). (b) the existence of a FDR for a system strongly coupled with its environment, here represented by an atom interacting with a quantum field. This is discussed in
Section 3.
Group B issues are (3) non-Markovian effects between two atoms, and (4) the nature and origin of quantum radiation. On (3) between pairs of atoms, we show the necessity of including a companion relation, the correlation-propagation relation (CPR) of the field describing how the correlations between the atoms are related to the propagation of their (retarded non-Markovian) mutual influence manifesting in the quantum field. It augments the FDR into a set of generalized matrix FDRs which capture completely the interaction between an atom and a quantum field at arbitrary coupling. On (4) We focus on how the quantum dynamics of the idf of the atom is related to emitted quantum radiation. Two noteworthy points are: it is quantum radiation, not classical, and it is emitted radiation, detectable at the far field zone a distance from the atom, not thermal radiance from a black body, as sensed by a uniformly accelerated detector (UAD) (the word ‘detector’ is used in the general relativity and relativistic quantum information community following [
15]. It usually refers to a source with internal degrees of freedom in motion. However, in radiation theory detector usually refers to the receiver at a distance from the source. In the present context, to avoid confusion, we shall reserve the term detector for the receiver and refer to the source as the atom, although we may keep the name of a Unruh-DeWitt [
16] detector and refer to a uniformly accelerated atom as UAD) in the Unruh effect. In fact we shall focus on the simplest possible set up, that of a stationary atom in a quantum field, thus there is no Unruh effect [
15] involved.
Quantum radiation is different by nature and origin (from quantum interference) from classical radiation, which can be viewed as the emitted quanta in the limiting condition of a coherent state. Quantum radiation from an accelerated electron under strong external electric field from a high power laser is described by Schützhold et al. [
17,
18]. Note the characteristics of quantum radiation from an accelerated electron—the photons are created in pairs (squeezed state) whose polarizations are perfectly correlated, engendering a nonthermal spectrum. They are very different from the Unruh effect proper, albeit both are quantum in nature. Recently Landulfo, Fulling and Matsas [
19] found a relation between Unruh thermal radiance in, and Larmor radiation emitted by, a uniformly accelerated charge, the latter can be seen as entirely built from zero-Rindler-energy modes, thus bridging the quantum and classical. As will be seen below, the conceptual scheme here will be at the level between the quantum and the semiclassical, namely, stochastic effects of vacuum fluctuations playing the role of quantum noise, and their backreaction on the idf of the atom. Technically, everything is done at the quantum field theory level. There is no need to introduce noise or stochasticity. In this paper we shall restrict our attention to stationary harmonic atoms, known as Unruh-DeWitt detectors in a relativistic context, not to moving charges.
One way to decipher whether there is quantum radiation is to calculate the stress–energy tensor of the quantum field. This quantity is of central importance in quantum effects of atom-optical and opto-mechanical systems such as dynamical Casimir effect [
20,
21] and quantum field theory in curved space [
22,
23,
24,
25]. Since this is a physical quantity defined in all space, if it vanishes then one can safely conclude there is no emitted radiation. This was done for a proof of the absence of emitted radiation from a UAD in a two-dimensional (2D) spacetime [
26], as first suggested by Grove [
27] and investigated by several groups of authors, e.g., [
28,
29,
30,
31,
32] (for a brief history of this theme and references in the first decade of its development, see, e.g., the Introduction of [
6], and for the general issues associated with UAD references [
33,
34].) However, it is not clear whether emitted quantum radiation exists in the four-dimensional (4D) case. In [
35], based on the perturbative argument for a two-level atom, Unruh and Wald argued that expected field energy does not increase from the viewpoint of an inertial observer. More detailed analysis for a harmonic atom with exact, analytical calculations [
36,
37] showed that an inertial observer in the far-field region at late times sees a net outward energy flux from the atom at its retarded position. The followup investigations [
38,
39] further show that this residual radiated energy seems to be related to the entanglement resulting from the decomposition of the Minkowski modes of the field into the Rindler modes in the right and the left wedges. In our companion paper [
40], we wish to offer a different perspective to understand quantum radiation from a uniformly accelerated atom by tracking down the energy flow with the help of the FDR and CPR. Here, as a prerequisite, since with a stationary atom, no radiation of any kind is expected, we use this simple fact to illustrate how the different contributing parts of energy sources add up to cancel each other. It is instructive to dissect this problem into parts so we can see the quantum and stochastic components of the atom, the field, and their interplay. We shall present the results of a calculation of the power delivered by different sources which add up to give us the anticipated result of net-zero energy in the far-field region. Namely, the emitted energy in the quantum radiation generated by the stochastic component in the dynamics of the system (the idf of the atom) induced by vacuum fluctuations of the quantum field is balanced by the vacuum fluctuations at all spatial points far away from the source. This is presented in
Section 5.
3. FDR in NEq Dynamics vs. Liner Response Theory
Since the fluctuation-dissipation relation (FDR) is the centerpiece in both sets of issues we indicated in the Introduction, namely, (A) the duality between vacuum fluctuations and quantum dissipation/quantum radiation reaction; and (B) the origin and nature of quantum radiation, as a sum of two parts (shown explicitly in the next section): one purely originating from the stochastic dynamics of the source (idf of the atom), and the other as the consequence of the interference between the radiated field from the source and the vacuum fluctuations of the field at the point of detection, it is useful to present a fuller description of the features, scopes and implications of FDRs.
Whilst FDR is traditionally presented in the context of linear response theory (LRT) [
48,
49,
50,
51,
52,
53] of systems in stationary configurations under weak disturbance, we feel that a new perspective of FDR versed in the context of nonequilibrium (NEq) dynamics is desirable to meet the new challenges of our time, when real time measurements of experimental results are becoming available which enable a broader scope in our understanding of the system’s properties. This is the approach we have adopted in treating a range of problems from atom-field interactions to quantum processes in black holes and the early universe. (For a glimpse of the scope of problems whose essences FDR can help to capture, see [
21,
54] and the Introduction of [
8,
9].)
3.1. Differences in the Set-Ups and the Main Features
Differences in the set-ups
Conventional FDR under LRT operates under the following assumptions: the system of interest (i) has been in equilibrium with the bath (say, in the Gibbs state) for a sufficiently long time that a stationary condition is established, and (ii) is subjected to a weak disturbance and its responses recorded. By contrast, in the nonequilibrium (NEq) formalism, the system can be in any arbitrary state, far from the thermal state at the bath temperature
or the equilibrium state the system finally settles in. Once the initial state of the system and the properties of the bath are given, for any specified system-bath interaction, we let go of both and let their interaction determine the outcome at late times. The ensuing dynamical evolution of the system under the influence of fluctuations from the bath can be captured by different methods in NEq dynamics of open quantum systems. The commonly used approaches include the quantum Langevin equation [
55] (for detector-field systems, see, e.g, [
36] and references therein) or influence functional methods [
56] (see [
57] and references therein). Fluctuations in the quantum field lead to quantum dissipation in the atom’s idf. After the system relaxes to a final equilibrium state their interlocked behavior is captured by the FDR.
Main features: FDR is an emergent relation in NEq
Since in LRT the FDR is formulated in terms of perturbative theory with respect to the equilibrium state of the system, it holds for all times. In the NEq case, the FDR in a strict sense is not available until the final equilibrium state is reached.
It might be useful at this point to make this statement: although LRT has a more restricted specified condition than NEq, they both belong to open system set-ups, which is formally different from the close system set-up of eigenvalue thermalization. For a depiction of the differences between the two formulations, see, e.g., the Introduction of [
58].
Weak coupling necessary for LRT, not required of NEq
Weak coupling is assumed in LRT to ensure the weak disturbance and validity of the perturbative treatment from an otherwise free system dynamics. No detailed knowledge of the system and the bath is need. Thus, similar to conventional thermodynamics, the formalism can be applied to a wide class of configurations as long as the aforementioned assumptions are met. For NEq dynamics, if the system and its coupling with the bath are linear in nature, Gaussian dynamics is exactly solvable for arbitrarily strong coupling strength as long as it stays within the realm of dynamical stability.
3.2. FDRs in System-Environment Interaction with Finite Coupling
Final equilibrated state not a Gibbs form
In contrast to LRT where the system remains in a thermal state at the bath temperature, in NEq dynamics, the system undergoes nonequilibrium evolution, and in most cases evolves to a final equilibrium state. In general, this equilibrium state is not a Gibbs (thermal) state unless the coupling strength between the system and the bath is vanishingly small. In the open-system conceptual framework, at finite coupling strength, there is a marked difference between equilibration and thermalization.
End state temperature in NEq not the same as the bath.
Since in the NEq formalism the final state does not necessarily assume a Gibbs form, the system temperature, identified from the equilibrated reduced density matrix of the system, is at best ‘effective’, because it depends on the details of the system and the bath parameters, far from being universal. Only in the vanishing coupling limit will the reduced system’s temperature approach the initial temperature of the bath. However, the bath has evolved away from its initial thermal configuration, albeit the difference is not so significant if the system has fewer degrees of freedom. Thus, only in this limit, where LRT operates, the system temperature, synonymous to the bath temperature, is independent of the system and the bath.
Different proportionality factor
In LRT, the proportionality factor in FDR depends on the system/bath temperature, while in the NEq formalism this factor depends on the initial temperature of the bath, which in general is not equal to the effective temperature of the final equilibrium state of the system, nor the temperature of the bath, identified in its later evolution.
3.3. FDR in a Dynamical Setting
In LRT, the FDR plays a rather passive, spectator role, relating the weak response of the system to an external agent’s disturbance. By contrast, in the NEQ formalism, FDR has a dynamical significance in that it ensures that the energy flow into the reduced system via the quantum fluctuations of the environment is balanced by the energy flow dispersed back to the environment in the form of quantum radiation. This energy rate or power balance shows how the FDR regulates the environment’s fluctuations and the system’s dissipation in a dynamical way. It also signifies the existence of an equilibrium state in this case.
In summary, owing to the requirement of self-consistency in the dynamics of the system and the bath, in the NEq theory the FDR at finite coupling strength cannot be given in an ad hoc manner. Existence of the FDR is conditional upon the system reaching equilibrium, which is not known a priori, but determined by the dynamics of the reduced system. Beside, At finite coupling strength if it exists, this equilibrium state is not by default the Gibbs thermal state.
5. Quantum Radiation from an Atom in 4D Minkowski Spacetime
We now present a calculation to show the relation between vacuum fluctuations, in the form of quantum noise, and quantum radiation and the role played by the FDR. Consider a static Unruh–DeWitt detector, whose internal degree of freedom (idf) is modeled by a simple harmonic oscillator, coupled to a massless scalar field (a note on the difference between an oscillator bath and a field bath with regard to quantum radiation. In the case of a bath made of harmonic oscillators, the system will transfer its energy to the bath through its coupling to the bath constituents. When the bath has an infinite number of constituents, the energy transferred from the system to the bath goes one way and does not return for a long, essentially infinite (Poincare) time. This is the dissipative effect in the system’s dynamics. If the bath oscillators occupy definite spatial points, e.g., forming a three-dimensional (3D) grid, and are coupled, then those closest to the atom will absorb the energy from the atom, and this energy will be transferred to the next closest neighbors spreading outwards. An observer at a finite distance from the atom will report on some of the bath oscillators getting excited when they absorb the energy and getting de-excited when the energy is transferred out. In this sense she see a (elastic) wave pattern of energy propagating away from the source, a situation resembling the quantum radiation from an atom in a field bath). We shall call this a harmonic atom, or simply the atom, to avoid confusion with a detector placed at a distance to measure emitted radiation. The field is initially in its thermal state, but the atom can assume any state. We assume the initial state of the total system is in a product form. Since such a prepared initial state is usually not an energy eigenstate of the combined atom-field system, there will be energy fluctuations and exchanges between the atom and the field. The field fluctuations will drive the idf of the atom into random motion, which in turn emits quantum radiation to the surrounding. Similar considerations have been implemented in the context of the moving mirror/dynamical Casimir effect problem [
59,
60,
61,
62,
63]. However, from the perspective of energy conservation, in particular if the field is initially in its vacuum state, then there is no energy reservoir that can sustain such radiated energy. Thus, we expect that there is no quantum radiation from a stationary atom. We shall reveal the energy budget of such a system and the role the FDRs play to balance the budget.
Earlier in [
8,
9,
58], we have studied the mechanism of energy flow, or power balance, from the viewpoint of the atom. There, we find that the reactive force from quantum radiation counters the motion of the atoms’ idf, driven by quantum fluctuations of the field. As the idfs gradually settle down, the system reaching an equilibrium state, the energy flow funneled in from the field fluctuations is balanced by the dissipated energy flow from the idf of the atom due to the frictional reactive force. The FDRs of the field and the atom ensure this balance. Here, focusing on the field, we explain how the energy balance can be reached even though no apparent conduit seems to exist to balance the radiated energy, thus highlighting the role of the FDRs in this ‘arrangement’.
5.1. Quantum Langevin Equation
From the simultaneous set of Heisenberg equations of motion of the internal degree of freedom
of the harmonic atom moving along a prescribed trajectory
and the massless scalar field
in
unbounded Minkowski space,
we find the formal solution of the field operator as
in which
e is the coupling constant,
, and
is the homogeneous solution to the wave Equation (2). The retarded Green’s function
of the free field, denoted by a subscript 0 to distinguish it from the interacting case, satisfies
Equation (
3) clearly shows that the total field at the observation point
x comprises of the vacuum fluctuations of the free field and the radiation field produced by the quantum dynamics of the atom (further explanation later).
Putting (
3) back to (
1), we arrive at
On the right hand side of this equation we see two source terms: The first term depicts vacuum field fluctuations
at the location
of the atom. It will induce stochastic motion in the internal degree of freedom of the atom. The second term contributing a nonlocal action in the equation of motion of the
operator accounts for radiation from the atom. When the configuration involves only a single atom in the massless scalar field, this nonlocal term reduces to two local contributions: one accounts for frequency renormalization and the other is a local damping term, such that (
5) takes a rather simple form
where
is the damping constant, whose inverse gives the time scale of relaxation, and
is the physical frequency, which includes the bare frequency
and the renormalization correction. Thus, the quantum radiation from the atom will introduce damping in the equation of motion of the idf of the atom, and this is the reactive force of quantum radiation we referred to earlier. Equation (
6) then says that the internal degree of freedom of the atom essentially behaves like a driven damped oscillator [
58,
64]—driven by the quantum fluctuations of the field, but is damped by the reactive force of quantum radiation.
The solution to (
5) or (
6) is given by
with
. Here, the homogeneous part
satisfies
The corresponding Green’s function
for the internal degree of freedom of the atom has a Fourier transform of the form
where the Fourier transformation of a function
is defined by
From (
7), we see the dynamics of the internal degree of freedom
of the atom contains two stochastic components: One comes from the homogeneous part of the solution, denoted by
, which depends on the initial conditions. This part is intrinsic in the sense that it is still present when the coupling is turned off, but will decay with time due to damping when the interaction is turned on. The other component is the inhomogeneous part in (
7), induced by the quantum fluctuations of the free field. The joint random motion of the idf, both of quantum origin, will give off quantum radiation to the atom’s surrounding, as can be seen from the second term on the right hand side of (
3).
If we want to investigate the properties of the field, Equation (
3) is an easier start. Since it is driven by the full
operator, we may substitute (
7) into (
3) and write the interacting field (
3) as
where
in the second term on the right hand side is the radiation field caused by the driven stochastic motion of the idf of the atom, and the third term on the right hand side, denoted by
is the transient radiation field from the homogeneous solution of
. The Hadamard function of the interacting field is readily given by
We see that on the right hand side the first term of (
13) results from the free field at the observation point, and the fourth term purely from the radiation field due to the induced stochastic motion of the internal degree of freedom. The second and third terms are of interest because they represent the interference between the free field and the radiation field at the observation point. The last term in (
14) does not contribute at late times because the homogeneous solution of the driven and damped oscillator exponentially decays with time, and for a given observation point, the radiation due to this component does not interfere with the local vacuum field and decreases with time.
Putting in the explicit expressions of
into (
13), we obtain
where
is the Hadamard function of the free field
and we have assumed that the initial state of the atom’s internal degree of freedom does not have cross correlation in the canonical variables.
The correlation function (
14) will be used to construct the stress-energy tensor of the interacting field
, based on which we will compute the late-time energy flow of the scalar field at an observation point far away from the atom.
5.2. A Stationary Atom
We consider the simplest case of an atom placed at a fixed location so that
is independent of time. Let
,
. For
t,
and
t,
,
, we can use the fluctuation–dissipation relations of the atom and the free field [
58]
in the expression
to greatly simplify the Hadamard function (
14) of the interacting field,
The last term in (
14) has been discarded. Application of the FDR in (
17) reduces the contribution purely from the radiation to a form that resembles those from the interference terms. This may not be a surprise on account that the late-time dynamics of the internal degree of freedom of the atom is predominantly governed by the quantum fluctuations of the free field in close proximity of the atom. A quick check shows that Equation (
18) satisfies the invariant property of the Hadamard function under the exchange of the coordinate points
and
. Also note that in (
16), we have assumed that the field is initially in a thermal state of temperature
, so the FDR of the free field is formulated for its initial state. By contrast, the FDR of the atom is obtained when the idf of the atom has relaxed to equilibrium after interacting with the field, despite their formal identity. In the case that the field is initially in a vacuum state, i.e.,
, just replace the factor
by the sign function
.
5.3. Stress-Energy Tensor of Field
The classical stress-energy tensor of a massless scalar field is given by
We will use the correlation function (
18) to find the expectation value of the normal-ordered stress-energy tensor operator
by
The radiated power far away from the atom is then given by
where
is the four-velocity of the (motion of the center of mass of the) atom at the retarded time
from the observation point
x, and
is a spacelike unit radial vector, so that the spatial distance
r between the observation point and the atom at the retarded time is given by
that is, the radius of the spherical shell passing through the observation point
with the origin at the retarded source point
of the atom. In the case of a static atom, the location
is fixed, so the four-velocity is a constant timelike unit vector along the time axis, whereby (
21) becomes
where
is the solid angle subtended over the spherical shell.
The coincidence limit of the derivatives
at late times is given by
Since we are interested in the flux at large distance from the atom, we keep only the far-field component in (
25), and obtain
Here we have used the FDR of the free field to re-write (
26). It then can be further reduced to
where we have used the property that
is odd in
,
even in
and
. Equation (
27) gives a vanishing result. Thus we find
that is, there is no net radiated energy at large distance from the atom at late times
.
5.4. Energy Flow Balance
This result is as expected. But this immediately prompts a question about how the radiated energy due to the stochastic motion of the internal degrees of freedom of the atom gets canceled? To track down the inner workings it will be more instructive to write the net radiated power (
28) as a sum of
and
, which are the energy flows associated with the second and the first terms inside the curly brackets, respectively, on the right hand side of (
27). They can further be reduced to
The radiation generated by the induced stochastic motion of the atom’s internal degree of freedom gives a power
at large distance from the atom at late times. This comes solely from the far-field component of the radiated field, and it gives an outward energy flow. However, we note that the radiated fields also interfere with the local vacuum fluctuations. This results, at infinity, in a net incoming flux of the same magnitude which cancels the aforementioned outgoing flux—an inertial observer in the distance will not measure any net energy flow. The generalized FDR, in particular the CPR, of the free field used in (
26) tells us that at an observation point far away from the atom, the radiation field is correlated with the vacuum field at that point in a nontrivial way, according to
Section 4 that their interference can concoct up an incoming flux to enable a perfect balance in the energy flow. Physically, this is a consequence of energy conservation. In particular, if the surrounding field is initially in the vacuum state, and if there is no external agent to supply energy, then there is no source/drain of energy to support a net energy flow in or out when the whole system settles down into equilibrium.
It will be more interesting to compare
and
with the power
dissipated by the atom and the power
supplied to the atom by the local vacuum fluctuations of the free field around the atom, at late times [
9,
58],
where we have used the FDR of the atom (
17), and the fact that
Equation (
31) explicitly shows that when the motion of the internal degrees of freedom of the atom reach equilibrium, the energy flow out of the atom due to the dissipative reactive force of quantum radiation is balanced by the power input from the local vacuum fluctuations of the free field. Therefore, comparison of Equations (
29)–(
31) tells us that this dissipated energy is radiated outward to infinity, i.e.,
. If we inadvertently ignore the contribution from the interference between the radiated field and the vacuum at the faraway location, then we will have a net energy output to infinity, which violates energy conservation. The interference contribution results in an inward energy flow which on one hand cancels the outgoing radiated energy and on the other hand replenishes the energy that is dumped into the atom from the vacuum field around it, that is,
. Thus the energy flow, from the viewpoint of either the atom or the field, is perfectly balanced at late times. Performing these cross-checks enables us to present an integrated and comprehensive picture of how the energy transfers from the atom to the surrounding field and back to the atom, meeting the stringent self-consistency constraint conditions ingrained in the FDRs-CPRs.