1. Introduction
Thanks to highly sensitive sensors, Fire Detection and Alarm Systems (FDAS) are used to identify fires at an early stage, which can be seen as a key part of the strategy to protect life and keep property safe from fires [
1]. One of the most critical techniques used in FDAS is smoke detection. It has been reported that a working smoke detector can reduce the risk of death from residential fires by 50% to 70% [
2]. There are two fire particle detection sensing modes, one ionisation and the other photoelectric. Ionisation smoke detectors are generally more responsive to smaller combustion products (<0.1 μm). On the other hand, photoelectric smoke sensors are more responsive to smaller combustion products (>0.1 μm) [
3,
4]. Ionisation smoke detectors have been phased out in many countries due to radioactivity, with photoelectric smoke sensors becoming the mainstream. Based on Festag’s investigations [
5], the false alarm ratio triggered by installed FDAS has been almost 90% in Germany in the last decade. From 2000 to 2014, over half of the fire alarms were false alarms in Great Britain, according to annual statistics compiled from Fire and Rescue Service records of incidents attended by fire and rescue authorities across Great Britain [
6]. The National Fire Protection Association (NFPA) reports that actual smoke alarm utilisation is more likely to be 92% in the United States, but almost 60% of home fire deaths have resulted from fires in properties with no smoke alarms (41%) or smoke alarms that did not work (16%) [
7]. According to this report, the leading cause of smoke alarms’ failure to operate was typically because of disconnected or non-working power sources. Power sources are often disabled because of unwanted alarms or false alarms. Frequent nuisance alarms can generate a dangerous sense of complacency, resulting in needless fatalities. Therefore, improving the reliability of photoelectric smoke detectors is very significant.
Common photoelectric smoke detectors consist of a near-infrared (NIR) light-emitting diode (LED) as a light source and a silicon photodiode (PD) as a light receptor. When no smoke is present, no light is detected by the photosensor. When smoke enters the chamber, the smoke particles partially absorb and partially scatter light in many directions, with some scattered light hitting the PD. The alarm goes off until the amount of incident light reaches a predetermined threshold. Unfortunately, other particles instead of smoke, including dust and water stream [
8,
9,
10], could have interfered with the intensity of scattered light to judge whether a fire had occurred.
The amount of light scattered by smoke is exceptionally complicated and is related to numerous factors, e.g., particle number density and size distribution, refractive index, light source wavelength, polarisation, and the angle between the light source and receiver. To reduce false alarms caused by non-fire particles, studies on the optical characteristics of smoke particles and other nuisance particles that change with angle and particle size have been conducted by the following authors. Loepfe et al. and Keller et al. measured angle- and polarisation-dependent light-scattering behaviours of fire aerosols from test fires of European Standard EN 54 and water vapour [
11,
12]. West et al. proposed the polarisation and scattering behaviours of mineral dust [
13]. Zhao [
14] measured the total scattering characteristics of fire smoke. Wang et al. proposed that the false alarms caused by interfering aerosols can be eliminated from multi-angle scattering detection [
15]. A practical application adopting multi-angle detection to eliminate false alarms caused by dust was described by Greenberg et al. [
16], who established a paraxial fire detection system in spacecraft to measure the surface area concentration and the volume concentration of the aerosols with a single-wavelength light source and dual received angles. Philipp et al. [
17] demonstrated the false alarm robustness of an optical sensor based on dual-wavelength light sources and multiple received angles to measure aerosols; they solved the problem of false alarms caused by dust, which is also the nuisance test specified in the UL 217 standard, but the interference of water mist cannot be effectively removed.
Recently, Shu Wang et al. [
18,
19] utilised the scattering intensity ratio of two different wavelength incident lights, which represents the Sauter Mean Diameter of aerosol particles under the theoretical deduction of the Mie scattering theory of homogeneous sphere particles [
20], to distinguish fire smoke and non-fire aerosols. These studies are very inspiring. However, the experiment setting was ideal, with measuring smoke particles generated by a monodisperse aerosol generator (MAG). Fire smoke is actually heterogeneous, and the scanning electron microscope images showed that some smoke particles have an approximate fractal structure [
21,
22]. The simple spherical hypothesis will increase the detection error in practical situations, which has also been found in our supplementary experiments in fire and interfering scenarios (especially the water vapour scenario). To distinguish non-spherical fire smoke from non-fire particles, some scholars have adopted models closer to the actual shape of soot particles. For example, Zhang [
23] used the Discrete Dipole Approximation (DDA) method to simulate the soot fractal agglomerates and demonstrated a significant difference between the DDA and spherical approximation for smoke scattering simulations. However, the scattering matrices measurement with polarised light that he used is unsuitable for engineering applications because its apparatus is too complex and bulky. A faster way to process received light signals for fire detection applications should be adopted to avoid increasing the response time.
Owing to the uncertainty of non-spherical characteristics of smoke particles on fire detection, this paper aims to introduce one more parameter to the work of Shu Wang et al., the extinction coefficient, to reduce uncertainties and resist false alarms. A Dual-Wavelength smoke detector measuring both light Scattering and Extinction (DWSE) is developed to reduce false alarms caused by dust and water vapour aerosols. First, through simplified spherical particle Mie scattering theory analysis, it is proved that the ratio of scattering intensity and the ratio of optical extinction of different wavelengths depends on the intrinsic particle size and refractive index of aerosol particles. In this way, both ratios can be utilised as fingerprints of the aerosols, and the supplementary measurement of extinction may somewhat eliminate the uncertainty brought by smoke particle shape. Then, three coefficients—the ratio of the scattering measures of two light sources , the ratio of the extinction measures of two light sources , and the ratio of the scattering measure to the extinction measure for one incident light —are proposed to distinguish smoke from dust and water mist. Next, to validate whether these three coefficients work for non-spherical fire smoke particles, the scattering simulation with the DDA method is made, and optimal detection angles for the two light sources are determined with real fire experiments. Finally, the proposed DWSE detector is verified with EN54 test fires.
Our study has two-fold contributions. First, it simultaneously measures the scattering and extinction of dual-wavelength light sources in one detector. The introduction of extinction has been proven to improve detection accuracy and reduce false alarms. Second, we introduce an alarm method with three coefficients , , and . Without complicated calculations of the Mie scattering or the DDA modelling of agglomerates, this alarm method is feasible for application in FDAS.
2. Theory
2.1. Mie Scattering and Extinction
Mie scattering theory was founded in 1908, as an analytical solution of Maxwell’s equations under the boundary conditions of monochromatic parallel light for an isotropic single dielectric sphere in a homogeneous medium. The Mie scattering coefficients are:
where
is the size parameter,
is the equivalent spherical diameter of the particle,
is the wavelength of incident light, and
is the complex refractive index [
24].
Equations (1) and (2) are known as Riccati–Bessel functions and are related to Bessel and Hankel functions [
25,
26]:
The scattering coefficient is:
Similarly, the extinction coefficient is:
The light intensity is as follows due to extinction:
where
is the light intensity of the light source,
is the distance from the light source, and
is derived from
.
Mie scattering theory is a precise description of the interaction between aerosol and particle. However, in this theoretical model, the optical scattering and extinction vary irregularly due to the coupled contributions of many factors, including particle shape and size, incident wavelength, etc. Therefore, using the Mie theory, it is difficult to examine the effect of a single factor for scattering. Thus, we will use a macroscopic scattering model called the “three regions” law to analyse the ratio of scattering intensity of two incident lights with different wavelengths, as well as the ratio of optical extinction.
2.2. The Ratio of Scattering Intensity
The “three regions” law was proposed by Gebhart in 2005 [
27]. It describes how the scattering intensity
varies with respect to particle size in the statistical measurement of aerosols. Let the intensity of light scattered by the unit volume of the spherical particle be:
where
is the scattering intensity due to a single amplitude and
is the observation angle from the emitter to the receiver. The relation between
,
, and
is shown in
Figure 1, and it can be divided into three regions:
(I) When , , ;
(II) When , , , which is proportional to the volume of the particle;
(III) When , , , which is proportional to the surface area of the particle.
, , and are the conversion factors for and in each region, , , and , respectively. From the continuity of the curve, it can be obtained that and , which means that and .
Since the aerosol is composed of particles with different sizes, let the distribution function be
, and then the scattering intensity of the aerosol is:
where
is the number concentration of the aerosol. The design of our proposed
DWSE learns from Shu Wang’s work [
19], picking the long wave
at region II and the short wave
at region III. Therefore, the scattering intensity can be expressed as:
where
is the volume concentration of the aerosol and
is the surface concentration of the aerosol. Taking the ratio of Equations (10) and (11), the following result can be obtained:
The concept of Sauter Mean Diameter (SMD)
is hereby introduced:
Therefore, . When the incident light wavelengths and the observation angles are fixed, is related to the refractive index . That is, the ratio of the scattering power with different incident light wavelengths depends on the average particle size and the refraction index.
2.3. The Ratio of Optical Extinction
For extinction, the parameter
in Equation (7) is related to Sauter Mean Diameter
, the particle number concentration
, and the wavelength
. This can be represented by the following formula [
28]:
where
is a dimensionless number. The ratio of the extinction coefficient can be defined as:
By substituting Equation (6), it can be obtained:
When the incident light wavelengths are fixed , the ratio is related to Mie coefficients ( and ). Mie coefficients are related to the particle size parameter and the refraction index. That is, the ratio of optical extinction with incident light wavelengths also depends on the average particle size and the refraction index.
To summarise, for our proposed DWSE, the wavelengths of two incident lights are fixed, and the ratio of scattering intensity and the ratio of optical extinction only depend on the intrinsic properties of the aerosol (the average particle size and the refractive index), which in theory can be used as characteristics to differentiate smoke aerosol and non-smoke aerosol.
4. Determination of Scattering Detection Angles
Both numerical simulations and experiments were carried out in this section. In the simulations, DDA-modelled fire smoke particles, paraffin aerosols, and two nuisance particles, i.e., fine water droplets and dust, were used to determine the optimal scattering detection angles. In the experiments, only paraffin aerosols and interfering particles were used since real fire is difficult to control, with it being unrealistic to conduct numerous fire experiments in this section. The real fire tests of EN54 were conducted in the next section for verification.
4.1. Calculation of Agglomerates Optical Properties by Discrete Dipole Approximation
Although paraffin aerosols can be regarded as spherical particles, real smoke particles are not spherical due to soot particles agglomerated and grown [
21]. Therefore, their scattering and extinction characteristics cannot be calculated directly by the Mie theory, and corresponding numerical calculation methods are required. The Discrete Dipole Approximation (DDA) method was used to determine more accurately the light scattering and extinction of soot aggregates and spheres derived from discrete element modelling. The DDA calculations were performed using open-source DDSCAT 7.3 code [
29]. To accomplish DDA computations, a number of parameters need to be determined.
The number of soot particles in an aggregate is given by:
where
is the radius of the individual soot particles,
is the radius of gyration, and
and
are the mass fractal dimension and fractal prefactor, respectively [
24]. According to Qiao’s research [
30], the radius of an individual soot particle was set to 30.8 nm. The coefficients
and
were determined to be 2.38 and 1.54, respectively, referring to Shu et al. [
21]. The number of soot particles
was specified as a maximum of 370, following a log-normal distribution with parameters
and
of 2.58 and 2.35, respectively. The refractive indices were set to 1.545 + 0.02i for both wavelengths.
4.2. Simulation
Paraffin aerosols, fine water droplets, and dust are all spherical particles, the scattering and extinction characteristics of which can be calculated by the Mie theory given the particle distribution. Therefore, measuring particle size distributions is the first step. The paraffin aerosols were produced by the aerosols generator (Aobosi ABS-Y02) used for fire detection testing according to EN 54, while the dust is ISO 12103-1, A2 fine test dust produced by Powder Technology Inc. The fine water droplets were generated by a household humidifier, which is reasonably similar to the actual scene. Particle size distributions of these particles were measured by a Malvern Spraytec system. This system measures spray droplets and sprays particle size distribution through laser diffraction. The refractive indices of paraffin aerosols, fine water droplets, and dust were set to 1.47, 1.33, and 1.51, respectively, according to the literature and databases, to ensure the accuracy of particle size distribution measurement [
31,
32,
33].
Figure 6 plots the particle distributions by volume of paraffin aerosols, fine water droplets, and dust, respectively. The volume-based median diameters (
) and Sauter diameters (
, SMD) of these particles calculated from measured particle size distributions are listed in
Table 1. Combined with
Figure 3 and
Table 1, there are apparent differences in particle size between aerosols, fine water droplets, and dust. The median particle size by volume of the aerosols is the smallest, 1.8 μm, while fine water droplets and dust are larger than 5 μm, which are also larger than the particle size of ordinary soot particles [
34]. In addition, it can be seen that the dust test data are roughly consistent with the standard distribution data provided by the manufacturer, as detailed in
Table 2.
The simulation results of paraffin aerosols, fine water droplets, dust, and DDA-modelled soot particles are presented in
Figure 7 and
Figure 8.
Figure 7 illustrates the simulated
of four different particles. It can be seen that
of agglomerates is significantly larger than the other three particles that can be regarded as spherical. As shown in
Figure 8, the relation curves of
and the scattering angles indicate that all particles have angular symmetry scattering characteristics to some extent except for the agglomerates, as predicted. The simulation results indicate that for all scattering angles, aerosols and agglomerates can be distinguished from fine water droplets and dust. In addition to smoke agglomerates, paraffin aerosols also need to be identified because they are used in the sensitivity test of EN 54.
4.3. Experiments
Although the simulation result is satisfactory, the actual situation still may have discrepancies with the simulation, which needs further confirmation by experiments. Three spherical particles (paraffin aerosols, fine water droplets, and dust) were tested. Particles were fed into the circumference centre within the DWSE detector through a unique tube to measure light intensities correctly. The background (, ), scattering, and extinction intensities without particles (, ) must be gauged before the test started. In each group of experiments, the scattering and extinction signals (, ) of the scattering angle from 20° to 160° were measured in steps of 5°.
Figure 9 shows an example of the results obtained during an angle determination test with paraffin aerosols, where the scattering angles were set to 90° for both wavelengths. The upper right plot (a) in
Figure 9 contains the time behaviour of the extinction and scattering signals from photodiodes in voltage. The paraffin aerosols generator was turned on at
s and emitted aerosols continuously and in a controlled manner into the detector so that the concentration rose linearly. At the same time, the extinction signals for both wavelengths reduced gradually due to the extinction of paraffin aerosols. The yellow line shows the voltage of the scattering channel for
and the green line shows the voltage of the scattering channel for
; they increased proportionally to the scattering as simulated. As can be seen from
Figure 9b–d, the calculated results of coefficients
for
,
for
, and
are 0.35477 ± 0.00024, 0.06820 ± 0.00004, and 0.8333 ± 0.0014, respectively.
Figure 10 represents an example of the results obtained during an angle determination test with fine water droplets, where the scattering angles were set to 90° for both wavelengths. As per
Figure 9, the upper right plots (a) in
Figure 10 present the time behaviour of the extinction and scattering signals in voltage. It can be seen that after the humidifier was turned on at
s, two scattering channels for
and
increased proportionally to the scattering in a similar nature to the aerosols. As shown in
Figure 10b–d, the calculated results of coefficients
for
,
for
, and
are 0.30962 ± 0.00028, 0.14442 ± 0.00011, and 1.0002 ± 0.0004, respectively.
Figure 11 presents an example of the results obtained during an angle determination test with the dust settled at a scattering angle of 90° for both wavelengths. Unlike
Figure 9 and
Figure 10, the design of the experimental device cannot increase the dust concentration linearly and can only be completed by reversing the timing sequence.
Figure 11 shows that the dust reached the highest value at the beginning of the test. The ventilation system was then activated, the dust concentration gradually decreased, the scattering signals also weakened, and the extinction signals gradually strengthened back to the initial value when there were no particles. According to
Figure 11b–d, the calculated results of coefficients
for
,
for
, and
are 0.54737 ± 0.00020, 0.09891 ± 0.00005, and 1.0907 ± 0.0005, respectively.
Figure 12 shows the experimental coefficients of extinction
of three different particles for
over
. The ratios of these particles are very close to each other, as shown in the simulation results in
Figure 7, and the significant uncertainty of the ratios cannot be neglected due to measurement errors. The results appear to demonstrate that this extinction detection has inadequate discrimination of aerosols, fine water droplets, and dust. It might be reasonable to suppose that distinguishing the above particles by relying only on extinction is not practical. The results suggest that
could be used as an auxiliary fire judgment.
Figure 13 provides the
of the four types of particles in log spacing for both wavelengths. It is noted that since the LED’s emission efficiency and the photodetector’s receiving efficiency are different between the two wavelengths, only the relative magnitude can be compared here rather than the absolute value. For
, since its wavelength is close to the size of these particles, the scattering properties vary with the angle and are not as symmetrical as
, which has a relatively shorter wavelength. Compared with the simulation results shown in
Figure 8, it seems that the discriminations are not as clear due to experimental error.
Relying solely on scattering or extinction is ineffective in distinguishing different particles. It is therefore necessary to combine scattering and extinction to detect these particles. In order to obtain the optimal scattering detection angles, the Euclidean distance of the four coefficients of each angle combination (
,
,
, and
) between two particles for an arbitrary scattering angle combination were calculated. The average Euclidean distance between the three particles was then shown in
Figure 14. The larger the Euclidean distance, the stronger the ability of this scattering detection angle to distinguish particles. The red grid indicates poor discrimination ability, while the dark green grid indicates strong discrimination ability, which is also the optimal detection angle required by this research. According to these guidelines,
scattering angles of 115° for and 60° for were selected as the scattering detection angles for the optimal
DWSE detector. Although other dark green grids may also be suitable, they should not impact the efficacy of our method and process.
5. Verification Fire Tests of EN 54
In order to verify if this optimal
DWSE detector could detect fire accurately and reduce false alarms caused by fine water droplets and dust, four types of EN 54 fire tests, presented in
Table 3, in a fire test chamber (10 m × 7 m × 4 m) were conducted with multiple times, as shown in
Figure 15 [
35,
36].
As displayed in
Figure 16, the coefficients of paraffin aerosols were set to unity for comparison since the aerosols were generated standardly. Comparing these coefficients shows that the
for each particle is the most effective basis for distinguishing between fire and nuisance sources, as shown in
Figure 16a, though the paraffin aerosol cannot be identified from nuisance particles. As represented in
Figure 16d, the coefficients
can also partially distinguish the fire from the interfering matters, especially for the paraffin aerosols, but the wood smouldering is close to dust, making the effect worse. Unfortunately, it is found that the
of test fires and
of nuisance particles for each wavelength vary in the same range, leading to an inconclusive judgement for this fire detection method. According to the above experimental results, and considering that the scattering signals are more sensitive than the extinction signals, the
can be used as a leading judgement, the
can be used as an auxiliary judgement to improve the accuracy, and, finally, verify
for
and
for
to ensure that there will be no false alarms.
In summary, the combination of scattering coefficients and and extinction coefficient is sufficient as a fire alarm criterion to distinguish between fire and interference sources.
6. Conclusions
Prior works have documented that false alarms caused by dust and fine water droplets should be reduced to ensure continuous smoke monitoring and fire protection. Philipp et al. [
15], for example, demonstrated an optical sensor based on dual-wavelength light sources with multiple received angles to detect smoke with no dust interference. However, fine water droplets can still cause false alarms with this optical sensor. In this study, we presented an improved Dual-Wavelength smoke detector measuring both light Scattering and Extinction (
DWSE) to reduce false alarms caused by fine water droplets and dust.
Two extinction-detection photodiodes were added to the improved DWSE detector to strengthen detection accuracy. It was found that fires can be distinguished from nuisance sources by comparing the calculated scattering coefficients and and extinction coefficient with optimal scattering angles of 115° for 940 nm and 60° for 470 nm. This study indicates that the DWSE detector and alarm method are suitable for smoke monitoring and fire protection because there is no complicated calculation of the Mie scattering or the DDA modelling of agglomerates. Fire scenarios might be inconsistent with verification experiments, but our results still provide theoretical possibilities for accomplishing real-world fire detection and reducing false alarms.
Some limitations of the research are worth noting. Firstly, the work on the optimal scattering angle needs to be better developed, and other combinations of relatively good scattering angles (dark green grids) need to be considered. Further research will be conducted to identify the best scattering angle for detecting smoke from actual fires, building upon the intriguing differences we observed in our study of other real fire tests and incidents. Another limitation is a better experimental chamber to facilitate quantitative measurements of physical parameters such as particle flow rate, thus making our coefficient determinations more accurate. It has only been proved that coefficients , , and can distinguish nuisance sources through simulation and limited experiments. However, we did not provide an intelligent fire alarm algorithm for the DWSE detector. The classification of different types of fire smoke needs to be considered in future work. Specifically, if enough dual-wavelength coefficients of different types of fire smoke can be accumulated, that is, to increase the amount of data, it will be helpful for the feasibility of intelligent identification and the improvement of detection accuracy.