International Journal of Environmental Research and Public Health

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16 pages, 3352 KiB

Open AccessArticle

The Release of Antimony from Mine Dump Soils in the Presence and Absence of Forest Litter

by Karolina Lewińska, Anna Karczewska, Marcin Siepak and Bernard Gałka

Int. J. Environ. Res. Public Health 2018, 15(12), 2631; https://doi.org/10.3390/ijerph15122631 - 24 Nov 2018

Cited by 16 | Viewed by 3379

Abstract

This study examined the changes in antimony (Sb) solubility in soils, using organic matter introduced with forest litter, in various moisture conditions. Soils containing 12.8–163 mg/kg Sb were taken from the top layers of dumps in former mining sites in the Sudetes, South-West [...] Read more.

This study examined the changes in antimony (Sb) solubility in soils, using organic matter introduced with forest litter, in various moisture conditions. Soils containing 12.8–163 mg/kg Sb were taken from the top layers of dumps in former mining sites in the Sudetes, South-West Poland. Soils were incubated for 90 days either in oxic or waterlogged conditions, with and without the addition of 50 g/kg of beech forest litter (FL). Water concentrations of Sb in some experimental treatments greatly exceeded the threshold values for good quality underground water and drinking water, and reached a maximum of 2.8 mg/L. The changes of Sb solubility caused by application of FL and prolonged waterlogging were, in various soils, highly divergent and in fact unpredictable based on the main soil properties. In some soils, the application of forest litter prompted the release of Sb from soil solid phase, while in the others it acted contradictorily. Soil waterlogging resulted, in most cases, in the increased release of Sb compared to oxic conditions, and this effect was enhanced by the addition of forest litter. However, in two soils the presence of forest litter counteracted the effects of waterlogging and diminished the quantities of released Sb. Full article

(This article belongs to the Special Issue Remediation and Analysis of Soil, Air, and Water Pollution)

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17 pages, 5016 KiB

Open AccessArticle

Variation of the Bacterial Community in the Rhizoplane Iron Plaque of the Wetland Plant Typha latifolia

by Haochun Chi, Lu Yang, Wenjing Yang, Yuanyuan Li, Ziwu Chen, Lige Huang, Yuanqing Chao, Rongliang Qiu and Shizhong Wang

Int. J. Environ. Res. Public Health 2018, 15(12), 2610; https://doi.org/10.3390/ijerph15122610 - 22 Nov 2018

Cited by 7 | Viewed by 3799

Abstract

The survival of wetland plants in iron, sulfur and heavy metals-rich mine tailing ponds has been commonly attributed to the iron plaque (IP) on the root surface that acts as a protective barrier. However, the contribution of bacteria potentially regulates the iron-sulfur cycle [...] Read more.

The survival of wetland plants in iron, sulfur and heavy metals-rich mine tailing ponds has been commonly attributed to the iron plaque (IP) on the root surface that acts as a protective barrier. However, the contribution of bacteria potentially regulates the iron-sulfur cycle and heavy metal exclusion at the root surface has not been studied in depth, particularly from a microbial ecology perspective. In this study, a pot experiment using Typha latifolia, a typical wetland plant, in non-polluted soil (NP) and tailing soil (T) was conducted. Samples from four zones, comprising non-rhizosphere soil (NR), rhizosphere soil (R) and internal (I) and external (E) layers of iron plaque, were collected from the NP and T and analyzed by 16S rRNA sequencing. Simpson index of the genus level showed greater diversities of bacterial community in the NP and its I zone is the most important part of the rhizosphere. PICRUSt predicted that the I zones in both NP and T harbored most of the functional genes. Specifically, functional genes related to sulfur relay and metabolism occurred more in the I zone in the T, whereas those related to iron acquisition and carbon and nitrogen circulation occurred more in the I zone in the NP. Analysis of dominant bacterial communities at genus level showed highest abundance of heavy metal resistant genus Burkholderia in the E zones in both soils, indicating that heavy metal resistance of Typha latifolia driven by Burkholderia mainly occurred at the external layer of IP. Moreover, many bacterial genera, such as Acidithiobacillus, Ferritrophicum, Thiomonas, Metallibacterium and Sideroxydans, involved in iron and sulfur metabolisms were found in the T and most showed higher abundance in the I zone than in the other zones. This work, as the first endeavor to separate the iron plaque into external and internal layers and investigate the variations of the bacterial communities therein, can provide an insight for further understanding the survival strategy of wetland plants, e.g., Typha latifolia, in extreme environment. Full article

(This article belongs to the Special Issue Remediation and Analysis of Soil, Air, and Water Pollution)

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14 pages, 1573 KiB

Open AccessArticle

Degradation of Triclosan and Carbamazepine in Two Agricultural and Garden Soils with Different Textures Amended with Composted Sewage Sludge

by Yanqiu Shao, Kai Yang, Rongchang Jia, Chao Tian and Ying Zhu

Int. J. Environ. Res. Public Health 2018, 15(11), 2557; https://doi.org/10.3390/ijerph15112557 - 14 Nov 2018

Cited by 13 | Viewed by 3630

Abstract

Composted sewage sludge (CSS) has been extensively used in agriculture and landscaping, offering a practical solution for waste disposal. However, some pharmaceutical and personal care products (PPCPs) like triclosan (TCS) and carbamazepine (CBZ) have restricted its land application. In this study, CSS was [...] Read more.

Composted sewage sludge (CSS) has been extensively used in agriculture and landscaping, offering a practical solution for waste disposal. However, some pharmaceutical and personal care products (PPCPs) like triclosan (TCS) and carbamazepine (CBZ) have restricted its land application. In this study, CSS was added to agricultural soil and garden soil at 0%, 5%, 10%, and 25% (w/w soil), and 4 mL of TCS and CBZ stock solution (1000 mg/L in methanol) was spiked into soil amended with CSS of each bottle to arrive at the concentration of 10 mg/kg. Samples were then collected after incubation for 120 days and analyzed for concentrations and half-life (t_1/2) of TCS and CBZ, and soil physicochemical properties, together with enzyme activities. The results showed that TCS was degraded completely during the incubation period. In contrast, only about 5.82–21.43% CBZ was degraded. CSS amendment inhibited TCS and CBZ degradation and prolonged t_1/2 compared to the control, and the t_1/2 of TCS and CBZ increased with CSS addition amount in all treatments except for CBZ in the garden soil amended with 10% CSS. Correlation studies showed a significantly positive relationship between t_1/2 of TCS and CBZ and total organic carbon (TOC), while a significantly negative relationship between t_1/2 of the two PPCPs and pH was observed. Alkaline phosphatase showed a significantly negative relationship with the C_t/C₀ of TCS in garden soil amended with 25% CSS and CBZ in the control. The urease activity was negatively correlated with the C_t/C₀ of TCS in 10% and 25% CSS treatments and CBZ in 10% CSS treatment for garden soil. Full article

(This article belongs to the Special Issue Remediation and Analysis of Soil, Air, and Water Pollution)

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20 pages, 1756 KiB

Open AccessArticle

Earthworms, Rice Straw, and Plant Interactions Change the Organic Connections in Soil and Promote the Decontamination of Cadmium in Soil

by Ali Mohamed Elyamine, Mohamed G. Moussa, Marwa A. Ismael, Jia Wei, Yuanyuan Zhao, Yupeng Wu and Chengxiao Hu

Int. J. Environ. Res. Public Health 2018, 15(11), 2398; https://doi.org/10.3390/ijerph15112398 - 29 Oct 2018

Cited by 33 | Viewed by 4725

Abstract

The joint effects of earthworms and crop straw on toxic metal speciation are not clear, and very limited information is available regarding the effects of their interaction on Cd mobility in Cd contaminated soil or in remediation processes involving plants. This study evaluated [...] Read more.

The joint effects of earthworms and crop straw on toxic metal speciation are not clear, and very limited information is available regarding the effects of their interaction on Cd mobility in Cd contaminated soil or in remediation processes involving plants. This study evaluated their impacts on Cd mobile form changes in soil and their effects on Cd uptake by plants. Treatments included both planted and unplanted-Cd-contaminated soil with or without rice straw and/or earthworms. The results revealed that earthworms, rice straw, and plant interactions change the Cd mobile forms in soil. The order of Cd concentration of different chemical forms was as follows: exchangeable > residual > bound to Fe-Mn oxide > bound to organic matter for earthworms, and exchangeable > bound to organic matter > residual > bound to Fe-Mn oxide for rice straw treatment, with a recovery rate of 96 ± 3%. The accumulation of Cd in plants increased in the presence of earthworms and decreased in the presence of rice straw. FT-IR spectra indicated that the degradation of rice straw increases C–O, C–O–H, C–H, and O–H functional groups which could complex with Cd ions. These findings highlighted that earthworms’ activities and crop straw can modify soil properties and structure and promote the remediation of heavy metal. This study suggests that the ecological context of remediation instead of being limiting on soil-earthworms-plant interaction, should integrate the natural resources forsaken which can provide a positive influence on both plant health and the remediation of heavy metal in contaminated soil. Full article

(This article belongs to the Special Issue Remediation and Analysis of Soil, Air, and Water Pollution)

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16 pages, 5839 KiB

Open AccessArticle

Silicon-Mediated Enhancement of Heavy Metal Tolerance in Rice at Different Growth Stages

by Fei Huang, Xiao-Hui Wen, Yi-Xia Cai and Kun-Zheng Cai

Int. J. Environ. Res. Public Health 2018, 15(10), 2193; https://doi.org/10.3390/ijerph15102193 - 8 Oct 2018

Cited by 58 | Viewed by 6668

Abstract

Silicon (Si) plays important roles in alleviating heavy metal stress in rice plants. Here we investigated the physiological response of rice at different growth stages under the silicon-induced mitigation of cadmium (Cd) and zinc (Zn) toxicity. Si treatment increased the dry weight of [...] Read more.

Silicon (Si) plays important roles in alleviating heavy metal stress in rice plants. Here we investigated the physiological response of rice at different growth stages under the silicon-induced mitigation of cadmium (Cd) and zinc (Zn) toxicity. Si treatment increased the dry weight of shoots and roots and reduced the Cd and Zn concentrations in roots, stems, leaves and grains. Under the stress of exposure to Cd and Zn, photosynthetic parameters including the chlorophyll content and chlorophyll fluorescence decreased, while the membrane permeability and malondialdehyde (MDA) increased. Catalase (CAT) and peroxidase (POD) activities increased under heavy metals stress, but superoxide dismutase (SOD) activities decreased. The magnitude of these Cd- and Zn-induced changes was mitigated by Si-addition at different growth stages. The available Cd concentration increased in the soil but significantly decreased in the shoots, which suggested that Si treatment prevents Cd accumulation through internal mechanisms by limiting Cd²⁺ uptake by the roots. Overall, the phenomena of Si-mediated alleviation of Cd and excess Zn toxicity in two rice cultivars could be due to the limitation of metal uptake and transport, resulting in an improvement in cell membrane integrity, photosynthetic performance and anti-oxidative enzyme activities after Si treatment. Full article

(This article belongs to the Special Issue Remediation and Analysis of Soil, Air, and Water Pollution)

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14 pages, 3645 KiB

Open AccessArticle

Ascorbate-Glutathione Cycle and Ultrastructural Analyses of Two Kenaf Cultivars (Hibiscus cannabinus L.) under Chromium Stress

by Lianmei Niu, Rang Cao, Jingquan Kang, Xu Zhang and Jinyin Lv

Int. J. Environ. Res. Public Health 2018, 15(7), 1467; https://doi.org/10.3390/ijerph15071467 - 11 Jul 2018

Cited by 11 | Viewed by 3260

Abstract

Kenaf (Hibiscus cannabinus L.) with high tolerance to chromium (Cr) can be used in the phytoremediation of chromium-contaminated soil. However, the mechanisms of chromium accumulation and tolerance in kenaf are still unclear. A hydroponic experiment was taken to screen two kenaf cultivars [...] Read more.

Kenaf (Hibiscus cannabinus L.) with high tolerance to chromium (Cr) can be used in the phytoremediation of chromium-contaminated soil. However, the mechanisms of chromium accumulation and tolerance in kenaf are still unclear. A hydroponic experiment was taken to screen two kenaf cultivars with Cr tolerance among nine kenaf cultivars via a tolerance index. This is first time the ascorbate-glutathione (AsA-GSH) cycle and chloroplast structural changes involved in Cr tolerance of two kenaf cultivars are explored. This study indicated that enhancement of chromium concentrations reduced nine kenaf growth rates and plant biomass. In addition, in all the nine cultivars, the roots had higher Cr accumulation than the shoots. Cr-tolerant cultivar Zhe70-3 with the maximum tolerant index had the significantly higher enzymatic activities of ascorbate peroxidase (APX), glutathione reductase (GR), dehydroascorbate reductase (DHAR) and mono- dehydroascorbate reductase (MDHAR) in non-enzymatic antioxidant system compared to Cr-sensitive cultivar Zhe77-1. In addition, higher GSH and AsA contents and lower damages of chloroplast ultrastructure were observed in Zhe70-3 under Cr treatment. In conclusion, Cr stress can cause less oxidative stress and destruction of chloroplast ultrastructure in Cr-tolerant cultivar Zhe70-3, and the AsA-GSH cycle may play a crucial role in kenaf Cr tolerance. Full article

(This article belongs to the Special Issue Remediation and Analysis of Soil, Air, and Water Pollution)

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13 pages, 3697 KiB

Open AccessArticle

Characterizing the Interaction between Antibiotics and Humic Acid by Fluorescence Quenching Method

by Runze Wang, Shengke Yang, Jie Fang, Zongzhou Wang, Yangyang Chen, Dan Zhang and Chunyan Yang

Int. J. Environ. Res. Public Health 2018, 15(7), 1458; https://doi.org/10.3390/ijerph15071458 - 10 Jul 2018

Cited by 32 | Viewed by 4094

Abstract

The method of Three-Dimensional Excitation Emission Matrix Fluorescence Spectrophotometer was used to identify the interaction mechanism between humic acid (HA) and antibiotics. The effects of antibiotic concentration, temperature, and pH on the bonding strength between HA and antibiotics were investigated. The results showed [...] Read more.

The method of Three-Dimensional Excitation Emission Matrix Fluorescence Spectrophotometer was used to identify the interaction mechanism between humic acid (HA) and antibiotics. The effects of antibiotic concentration, temperature, and pH on the bonding strength between HA and antibiotics were investigated. The results showed that with the increase of antibiotics concentration, the quenching effect on HA was enhanced. The quenching of HA by both oxytetracycline (OTC) and sulfadiazine (SD) is a single static quenching of the complexes, and the interaction forces are mainly a hydrogen bond and the van der Waals force. The quenching constant K_svOTC > K_svSD and the binding constant K_bOTC > K_bSD, indicates that HA has a more obvious quenching effect on OTC. The K_b of HA by OTC ranged from 3.223 × 10³ to 12.784 × 10³ L·mol⁻¹ in the range of 298 K to 313 K, while the K_b of HA by SD ranged from 2.051 × 10³ to 5.533 × 10³ L·mol⁻¹. With the increase of temperature, the quenching constant K_sv and binding constant K_b of both OTC and SD by HA gradually decrease, and the low temperature is beneficial to the interaction. The composite of OTC and HA is more stable than SD. Under neutral alkaline conditions, both OTC and SD had the strongest quenching effect on HA, and the resulting complex was the most stable. However, the K_sv and Kb of HA by OTC were greater than SD in the pH range of the experiment and the pH effect on quenching of HA by OTC (K_sv) was greater than that of SD. Full article

(This article belongs to the Special Issue Remediation and Analysis of Soil, Air, and Water Pollution)

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14 pages, 5697 KiB

Open AccessArticle

Source Identification and Apportionment of Trace Elements in Soils in the Yangtze River Delta, China

by Shuai Shao, Bifeng Hu, Zhiyi Fu, Jiayu Wang, Ge Lou, Yue Zhou, Bin Jin, Yan Li and Zhou Shi

Int. J. Environ. Res. Public Health 2018, 15(6), 1240; https://doi.org/10.3390/ijerph15061240 - 12 Jun 2018

Cited by 34 | Viewed by 5849

Abstract

Trace elements pollution has attracted a lot of attention worldwide. However, it is difficult to identify and apportion the sources of multiple element pollutants over large areas because of the considerable spatial complexity and variability in the distribution of trace elements in soil. [...] Read more.

Trace elements pollution has attracted a lot of attention worldwide. However, it is difficult to identify and apportion the sources of multiple element pollutants over large areas because of the considerable spatial complexity and variability in the distribution of trace elements in soil. In this study, we collected total of 2051 topsoil (0–20 cm) samples, and analyzed the general pollution status of soils from the Yangtze River Delta, Southeast China. We applied principal component analysis (PCA), a finite mixture distribution model (FMDM), and geostatistical tools to identify and quantitatively apportion the sources of seven kinds of trace elements (chromium (Cr), cadmium (Cd), mercury (Hg), copper (Cu), zinc (Zn), nickel (Ni), and arsenic (As)) in soil. The PCA results indicated that the trace elements in soil in the study area were mainly from natural, multi-pollutant and industrial sources. The FMDM also fitted three sub log-normal distributions. The results from the two models were quite similar: Cr, As, and Ni were mainly from natural sources caused by parent material weathering; Cd, Cu, and Zu were mainly from mixed sources, with a considerable portion from anthropogenic activities such as traffic pollutants, domestic garbage, and agricultural inputs, and Hg was mainly from industrial wastes and pollutants. Full article

(This article belongs to the Special Issue Remediation and Analysis of Soil, Air, and Water Pollution)

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18 pages, 1437 KiB

Open AccessArticle

Adsorption Performance Analysis of Alternative Reactive Media for Remediation of Aquifers Affected by Heavy Metal Contamination

by Antonio Molinari, Celia Margarita Mayacela Rojas, Amerigo Beneduci, Adalgisa Tavolaro, Maria Fernanda Rivera Velasquez and Carmine Fallico

Int. J. Environ. Res. Public Health 2018, 15(5), 980; https://doi.org/10.3390/ijerph15050980 - 14 May 2018

Cited by 8 | Viewed by 3940

Abstract

A series of experimental batch tests has been carried out with the aim of improving the knowledge of fundamental processes related to the fate and behavior of heavy metals that can be of environmental concern in groundwater. The analysis of contaminants (i.e., Cu, [...] Read more.

A series of experimental batch tests has been carried out with the aim of improving the knowledge of fundamental processes related to the fate and behavior of heavy metals that can be of environmental concern in groundwater. The analysis of contaminants (i.e., Cu, Zn, Cd and Pb) dynamics in different environmental compartments is specifically addressed by comparing the removal efficiencies of different types of reactive materials, three natural (i.e., vegetal fibers, natural limestone and natural zeolite) and one synthetic (i.e., synthetic zeolite). Results stemming from these reactive media has been compared with the outcomes related to the same test performed using zero valent iron which is the reactant usually employed for heavy metals remediation. All tested reactants exhibited important removal percentages, even larger than 90% in most cases, achieved in a contact time ranging between about 12 h and slightly longer than a day (i.e., 30 h). Maximum adsorption percentages are observed for pH ranging between 4 and 8 for all tested materials and contaminants. Our findings provided relevant evidence, to both researchers and technicians, on the competitiveness of the explored alternative mediums with respect to the classical reactants usually employed for heavy metals remediation. Full article

(This article belongs to the Special Issue Remediation and Analysis of Soil, Air, and Water Pollution)

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18 pages, 1864 KiB

Open AccessArticle

Biocapture of CO₂ by Different Microalgal-Based Technologies for Biogas Upgrading and Simultaneous Biogas Slurry Purification under Various Light Intensities and Photoperiods

by Pengfei Guo, Yuejin Zhang and Yongjun Zhao

Int. J. Environ. Res. Public Health 2018, 15(3), 528; https://doi.org/10.3390/ijerph15030528 - 15 Mar 2018

Cited by 24 | Viewed by 4288

Abstract

Co-cultivation of microalgae and microbes for pollutant removal from sewage is considered as an effective wastewater treatment method. The aim of this study is to screen the optimal photoperiod, light intensity and microalgae co-cultivation method for simultaneously removing nutrients in biogas slurry and [...] Read more.

Co-cultivation of microalgae and microbes for pollutant removal from sewage is considered as an effective wastewater treatment method. The aim of this study is to screen the optimal photoperiod, light intensity and microalgae co-cultivation method for simultaneously removing nutrients in biogas slurry and capturing CO₂ in biogas. The microalgae–fungi pellets are deemed to be a viable option because of their high specific growth rate and nutrient and CO₂removal efficiency under the photoperiod of 14 h light:10 h dark. The order of both the biogas slurry purification and biogas upgrading is ranked the same, that is Chlorella vulgaris–Ganoderma lucidum > Chlorella vulgaris–activated sludge > Chlorella vulgaris under different light intensities. For all cultivation methods, the moderate light intensity of 450 μmol m⁻² s⁻¹ is regarded as the best choice. This research revealed that the control of photoperiod and light intensity can promote the biological treatment process of biogas slurry purification and biogas upgrading using microalgal-based technology. Full article

(This article belongs to the Special Issue Remediation and Analysis of Soil, Air, and Water Pollution)

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1611 KiB

Open AccessArticle

Aerobic Biodegradation Characteristic of Different Water-Soluble Azo Dyes

by Shixiong Sheng, Bo Liu, Xiangyu Hou, Bing Wu, Fang Yao, Xinchun Ding and Lin Huang

Int. J. Environ. Res. Public Health 2018, 15(1), 35; https://doi.org/10.3390/ijerph15010035 - 26 Dec 2017

Cited by 16 | Viewed by 4249

Abstract

This study investigated the biodegradation performance and characteristics of Sudan I and Acid Orange 7 (AO7) to improve the biological dye removal efficiency in wastewater and optimize the treatment process. The dyes with different water-solubility and similar molecular structure were biologically treated under [...] Read more.

This study investigated the biodegradation performance and characteristics of Sudan I and Acid Orange 7 (AO7) to improve the biological dye removal efficiency in wastewater and optimize the treatment process. The dyes with different water-solubility and similar molecular structure were biologically treated under aerobic condition in parallel continuous-flow mixed stirred reactors. The biophase analysis using microscopic examination suggested that the removal process of the two azo dyes is different. Removal of Sudan I was through biosorption, since it easily assembled and adsorbed on the surface of zoogloea due to its insolubility, while AO7 was biodegraded incompletely and bioconverted, the AO7 molecule was decomposed to benzene series and inorganic ions, since it could reach the interior area of zoogloea due to the low oxidation-reduction potential conditions and corresponding anaerobic microorganisms. The transformation of NH₃-N, SO₄²⁻ together with the presence of tryptophan-like components confirm that AO7 can be decomposed to non-toxic products in an aerobic bioreactor. This study provides a theoretical basis for the use of biosorption or biodegradation mechanisms for the treatment of different azo dyes in wastewater. Full article

(This article belongs to the Special Issue Remediation and Analysis of Soil, Air, and Water Pollution)

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28045 KiB

Open AccessArticle

Spatiotemporal Variations and Driving Factors of Air Pollution in China

by Dongsheng Zhan, Mei-Po Kwan, Wenzhong Zhang, Shaojian Wang and Jianhui Yu

Int. J. Environ. Res. Public Health 2017, 14(12), 1538; https://doi.org/10.3390/ijerph14121538 - 8 Dec 2017

Cited by 42 | Viewed by 7021

Abstract

In recent years, severe and persistent air pollution episodes in China have drawn wide public concern. Based on ground monitoring air quality data collected in 2015 in Chinese cities above the prefectural level, this study identifies the spatiotemporal variations of air pollution and [...] Read more.

In recent years, severe and persistent air pollution episodes in China have drawn wide public concern. Based on ground monitoring air quality data collected in 2015 in Chinese cities above the prefectural level, this study identifies the spatiotemporal variations of air pollution and its associated driving factors in China using descriptive statistics and geographical detector methods. The results show that the average air pollution ratio and continuous air pollution ratio across Chinese cities in 2015 were 23.1 ± 16.9% and 16.2 ± 14.8%. The highest levels of air pollution ratio and continuous air pollution ratio were observed in northern China, especially in the Bohai Rim region and Xinjiang province, and the lowest levels were found in southern China. The average and maximum levels of continuous air pollution show distinct spatial variations when compared with those of the continuous air pollution ratio. Monthly changes in both air pollution ratio and continuous air pollution ratio have a U-shaped variation, indicating that the highest levels of air pollution occurred in winter and the lowest levels happened in summer. The results of the geographical detector model further reveal that the effect intensity of natural factors on the spatial disparity of the air pollution ratio is greater than that of human-related factors. Specifically, among natural factors, the annual average temperature, land relief, and relative humidity have the greatest and most significant negative effects on the air pollution ratio, whereas human factors such as population density, the number of vehicles, and Gross Domestic Product (GDP) witness the strongest and most significant positive effects on air pollution ratio. Full article

(This article belongs to the Special Issue Remediation and Analysis of Soil, Air, and Water Pollution)

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1027 KiB

Open AccessArticle

OMI and Ground-Based In-Situ Tropospheric Nitrogen Dioxide Observations over Several Important European Cities during 2005–2014

by Spiru Paraschiv, Daniel-Eduard Constantin, Simona-Lizica Paraschiv and Mirela Voiculescu

Int. J. Environ. Res. Public Health 2017, 14(11), 1415; https://doi.org/10.3390/ijerph14111415 - 20 Nov 2017

Cited by 24 | Viewed by 5160

Abstract

In this work we present the evolution of tropospheric nitrogen dioxide (NO₂) content over several important European cities during 2005–2014 using space observations and ground-based in-situ measurements. The NO₂ content was derived using the daily observations provided by the Ozone [...] Read more.

In this work we present the evolution of tropospheric nitrogen dioxide (NO₂) content over several important European cities during 2005–2014 using space observations and ground-based in-situ measurements. The NO₂ content was derived using the daily observations provided by the Ozone Monitoring Instrument (OMI), while the NO₂ volume mixing ratio measurements were obtained from the European Environment Agency (EEA) air quality monitoring stations database. The European cities selected are: Athens (37.98° N, 23.72° E), Berlin (52.51° N, 13.41° E), Bucharest (44.43° N, 26.10° E), Madrid (40.38° N, 3.71° W), Lisbon (38.71° N, 9.13° W), Paris (48.85° N, 2.35° E), Rome (41.9° N, 12.50° E), and Rotterdam (51.91° N, 4.46° E). We show that OMI NO₂ tropospheric column data can be used to assess the evolution of NO₂ over important European cities. According to the statistical analysis, using the seasonal variation, we found good correlations (R > 0.50) between OMI and ground-based in-situ observations for all of the cities presented in this work. Highest correlation coefficients (R > 0.80) between ground-based monitoring stations and OMI observations were calculated for the cities of Berlin, Madrid, and Rome. Both types of observations, in-situ and remote sensing, show an NO₂ negative trend for all of locations presented in this study. Full article

(This article belongs to the Special Issue Remediation and Analysis of Soil, Air, and Water Pollution)

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1031 KiB

Open AccessArticle

Occurrences of Organochlorine Pesticides along the Course of the Buffalo River in the Eastern Cape of South Africa and Its Health Implications

by Abdulrazaq Yahaya, Omobola O. Okoh, Anthony I. Okoh and Abiodun O. Adeniji

Int. J. Environ. Res. Public Health 2017, 14(11), 1372; https://doi.org/10.3390/ijerph14111372 - 10 Nov 2017

Cited by 49 | Viewed by 6910

Abstract

Most organochlorine pesticides (OCPs) which are increasingly used in agriculture and industry are not biodegradable and thereby persist in the environment for a very long period of time. They are capable of negatively impacting the health of humans and biota when present in [...] Read more.

Most organochlorine pesticides (OCPs) which are increasingly used in agriculture and industry are not biodegradable and thereby persist in the environment for a very long period of time. They are capable of negatively impacting the health of humans and biota when present in a higher concentration than recommended. This study evaluated the concentrations of 17 OCPs in surface water samples collected from six sampling sites along the course of the Buffalo River in Eastern Cape, South Africa, between December 2015 and May 2016. The samples were subjected to solvent extraction, followed by florisil clean up, and analyzed using gas chromatography coupled with an electron capture detector. The individual concentrations of OCPs detected ranged from <LOD to 4403 ng/L in summer and <LOD to 313 ng/L in autumn. The levels of OCPs in the study area were generally above the United State Environmental Protection Agency (USEPA) limit of 100 ng/L in all the sampling locations in the two seasons. The cancer risk assessment values were below the permissible limit of the 10⁻⁶ level, although the life average daily dose were slightly above the USEPA maximum limits of 10⁻⁴. Therefore, there is a need for the adequate regulation of agrochemical storage, use, and disposal in this province and other parts of South Africa. Full article

(This article belongs to the Special Issue Remediation and Analysis of Soil, Air, and Water Pollution)

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Review

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16 pages, 1015 KiB

Open AccessReview

Heavy Metal and Metalloid Pollution of Soil, Water and Foods in Bangladesh: A Critical Review

by M. Mominul Islam, Md. Rezaul Karim, Xin Zheng and Xiaofang Li

Int. J. Environ. Res. Public Health 2018, 15(12), 2825; https://doi.org/10.3390/ijerph15122825 - 11 Dec 2018

Cited by 127 | Viewed by 20284

Abstract

Bangladesh is a densely populated developing country. Both industrialization and geological sources have caused widespread heavy metal and metalloid pollution in Bangladesh, which is now posing substantial threats to the local people. In this review, we carried out one of the most exhaustive [...] Read more.

Bangladesh is a densely populated developing country. Both industrialization and geological sources have caused widespread heavy metal and metalloid pollution in Bangladesh, which is now posing substantial threats to the local people. In this review, we carried out one of the most exhaustive literature analyses on the current status of Bangladesh heavy metal and metalloid pollution, covering water, soil, and foods. Analysis showed that soils near high traffic and industrial areas contain high concentrations of heavy metals and metalloids. Agricultural land and vegetables in sewage-irrigated areas were also found to be heavy metal- and metalloid-contaminated. River water, sediment, and fish from the Buriganga, Turag, Shitalakhya, and Karnaphuli rivers are highly contaminated with cadmium (Cd), lead (Pb), and chromium (Cr). Particularly, groundwater arsenic (As) pollution associated with high geological background levels in Bangladesh is well reported and is hitherto the largest mass poisoning in the world. Overall, the contamination levels of heavy metals and metalloids vary among the cities, with industrial areas being most polluted. In all, this review provides a quantitative identification of the As, Pb, Cd, and Cr contamination hotspots in Bangladesh based on the literature, which may be useful to environmental restorationists and local policy makers. Full article

(This article belongs to the Special Issue Remediation and Analysis of Soil, Air, and Water Pollution)

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1887 KiB

Open AccessReview

Microbial and Plant-Assisted Bioremediation of Heavy Metal Polluted Environments: A Review

by Omena Bernard Ojuederie and Olubukola Oluranti Babalola

Int. J. Environ. Res. Public Health 2017, 14(12), 1504; https://doi.org/10.3390/ijerph14121504 - 4 Dec 2017

Cited by 769 | Viewed by 40373

Abstract

Environmental pollution from hazardous waste materials, organic pollutants and heavy metals, has adversely affected the natural ecosystem to the detriment of man. These pollutants arise from anthropogenic sources as well as natural disasters such as hurricanes and volcanic eruptions. Toxic metals could accumulate [...] Read more.

Environmental pollution from hazardous waste materials, organic pollutants and heavy metals, has adversely affected the natural ecosystem to the detriment of man. These pollutants arise from anthropogenic sources as well as natural disasters such as hurricanes and volcanic eruptions. Toxic metals could accumulate in agricultural soils and get into the food chain, thereby becoming a major threat to food security. Conventional and physical methods are expensive and not effective in areas with low metal toxicity. Bioremediation is therefore an eco-friendly and efficient method of reclaiming environments contaminated with heavy metals by making use of the inherent biological mechanisms of microorganisms and plants to eradicate hazardous contaminants. This review discusses the toxic effects of heavy metal pollution and the mechanisms used by microbes and plants for environmental remediation. It also emphasized the importance of modern biotechnological techniques and approaches in improving the ability of microbial enzymes to effectively degrade heavy metals at a faster rate, highlighting recent advances in microbial bioremediation and phytoremediation for the removal of heavy metals from the environment as well as future prospects and limitations. However, strict adherence to biosafety regulations must be followed in the use of biotechnological methods to ensure safety of the environment. Full article

(This article belongs to the Special Issue Remediation and Analysis of Soil, Air, and Water Pollution)

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