Atmosphere

1175 KiB

Open AccessArticle

A High Resolution Spatiotemporal Model for In-Vehicle Black Carbon Exposure: Quantifying the In-Vehicle Exposure Reduction Due to the Euro 5 Particulate Matter Standard Legislation

by Luc Dekoninck and Luc Int Panis

Atmosphere 2017, 8(11), 230; https://doi.org/10.3390/atmos8110230 - 22 Nov 2017

Cited by 5 | Viewed by 7132

Abstract

Several studies have shown that a significant amount of daily air pollution exposure is inhaled during trips. In this study, car drivers assessed their own black carbon exposure under real-life conditions (223 h of data from 2013). The spatiotemporal exposure of the car [...] Read more.

Several studies have shown that a significant amount of daily air pollution exposure is inhaled during trips. In this study, car drivers assessed their own black carbon exposure under real-life conditions (223 h of data from 2013). The spatiotemporal exposure of the car drivers is modeled using a data science approach, referred to as “microscopic land-use regression” (µLUR). In-vehicle exposure is highly dynamical and is strongly related to the local traffic dynamics. An extensive set of potential covariates was used to model the in-vehicle black carbon exposure in a temporal resolution of 10 s. Traffic was retrieved directly from traffic databases and indirectly by attributing the trips through a noise map as an alternative traffic source. Modeling by generalized additive models (GAM) shows non-linear effects for meteorology and diurnal traffic patterns. A fitted diurnal pattern explains indirectly the complex diurnal variability of the exposure due to the non-linear interaction between traffic density and distance to the preceding vehicles. Comparing the strength of direct traffic attribution and indirect noise map-based traffic attribution reveals the potential of noise maps as a proxy for traffic-related air pollution exposure. An external validation, based on a dataset gathered in 2010–2011, quantifies the exposure reduction inside the vehicles at 33% (mean) and 50% (median). The EU PM Euro 5 PM emission standard (in force since 2009) explains the largest part of the discrepancy between the measurement campaign in 2013 and the validation dataset. The µLUR methodology provides a high resolution, route-sensitive, seasonal and meteorology-sensitive personal exposure estimate for epidemiologists and policy makers. Full article

(This article belongs to the Special Issue Carbonaceous Aerosols in Atmosphere)

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2411 KiB

Open AccessArticle

Atmospheric Processing and Variability of Biological Ice Nucleating Particles in Precipitation at Opme, France

by Glwadys Pouzet, Elodie Peghaire, Maxime Aguès, Jean-Luc Baray, Franz Conen and Pierre Amato

Atmosphere 2017, 8(11), 229; https://doi.org/10.3390/atmos8110229 - 21 Nov 2017

Cited by 16 | Viewed by 5294

Abstract

Atmospheric ice nucleating particles (INPs) contribute to initiate precipitation. In particular, biological INPs act at warmer temperatures than other types of particles (>−10 °C) therefore potentially defining precipitation distribution. Here, in order to identify potential environmental drivers in the distribution and fate of [...] Read more.

Atmospheric ice nucleating particles (INPs) contribute to initiate precipitation. In particular, biological INPs act at warmer temperatures than other types of particles (>−10 °C) therefore potentially defining precipitation distribution. Here, in order to identify potential environmental drivers in the distribution and fate of biological INPs in the atmosphere, we conducted a mid-term study of the freezing characteristics of precipitation. A total of 121 samples were collected during a period of >1.5 years at the rural site of Opme (680 m a.s.l. (above sea level), France). INP concentration ranged over two orders of magnitude at a given temperature depending on the sample; there were <1 INPs mL⁻¹ at ≥−5 °C, ~0.1 to 10 mL⁻¹ between −5 °C and −8 °C, and ~1 to 100 mL⁻¹ at colder temperatures. The data support the existence of an intimate natural link between biological INPs and hydrological cycles. In addition, acidification was strongly correlated with a decrease of the freezing characteristics of the samples, suggesting that human activities impact the role of INPs as triggers of precipitation. Water isotope ratio measurements and statistical comparison with aerosol and cloud water data confirmed some extent of INP partitioning in the atmosphere, with the INPs active at the warmest temperatures tending to be more efficiently precipitated. Full article

(This article belongs to the Special Issue Atmospheric Aerosol Composition and its Impact on Clouds)

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3055 KiB

Open AccessArticle

Optical Properties of Biomass Burning Aerosols: Comparison of Experimental Measurements and T-Matrix Calculations

by Samin Poudel, Marc N. Fiddler, Damon Smith, K. M. Flurchick and Solomon Bililign

Atmosphere 2017, 8(11), 228; https://doi.org/10.3390/atmos8110228 - 21 Nov 2017

Cited by 13 | Viewed by 6802

Abstract

The refractive index (RI) is an important parameter in describing the radiative impacts of aerosols. It is important to constrain the RI of aerosol components, since there is still significant uncertainty regarding the RI of biomass burning aerosols. Experimentally measured extinction cross-sections, scattering [...] Read more.

The refractive index (RI) is an important parameter in describing the radiative impacts of aerosols. It is important to constrain the RI of aerosol components, since there is still significant uncertainty regarding the RI of biomass burning aerosols. Experimentally measured extinction cross-sections, scattering cross-sections, and single scattering albedos for white pine biomass burning (BB) aerosols under two different burning and sampling conditions were modeled using T-matrix theory. The refractive indices were extracted from these calculations. Experimental measurements were conducted using a cavity ring-down spectrometer to measure the extinction, and a nephelometer to measure the scattering of size-selected aerosols. BB aerosols were obtained by burning white pine using (1) an open fire in a burn drum, where the aerosols were collected in distilled water using an impinger, and then re-aerosolized after several days, and (2) a tube furnace to directly introduce the BB aerosols into an indoor smog chamber, where BB aerosols were then sampled directly. In both cases, filter samples were also collected, and electron microscopy images were used to obtain the morphology and size information used in the T-matrix calculations. The effective radius of the particles collected on filter media from the open fire was approximately 245 nm, whereas it was approximately 76 nm for particles from the tube furnace burns. For samples collected in distilled water, the real part of the RI increased with increasing particle size, and the imaginary part decreased. The imaginary part of the RI was also significantly larger than the reported values for fresh BB aerosol samples. For the particles generated in the tube furnace, the real part of the RI decreased with particle size, and the imaginary part was much smaller and nearly constant. The RI is sensitive to particle size and sampling method, but there was no wavelength dependence over the range considered (500–680 nm). Our values for the RI of fresh (white pine) biomass burning aerosols ranged from 1.33 + i0.008 to 1.74 + i0.008 for 200-nm, 300-nm, and 400-nm diameter particles. These are within the range of RI values in the most recent study conducted during the Fire Laboratory at Missoula Experiments (FLAME I and II), which were 1.55 to 1.80 for the real part, and 0.01–0.50 for the imaginary part, for fresh BB aerosols with diameters of 200–570 nm. There is no clear trend on the dependence of the RI values on particle size. The RI values derived from measurements of aerosols produced from the combustion of hydrocarbons and diesel cannot be used for BB aerosols. Full article

(This article belongs to the Special Issue Aerosol Optical Properties: Models, Methods & Measurements)

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556 KiB

Open AccessArticle

Evaluation and Inter-Comparison of Oxygen-Based OC-EC Separation Methods for Radiocarbon Analysis of Ambient Aerosol Particle Samples

by Katrin Zenker, Matthias Vonwiller, Sönke Szidat, Giulia Calzolai, Martina Giannoni, Vera Bernardoni, Aleksandra D. Jedynska, Bas Henzing, Harro A. J. Meijer and Ulrike Dusek

Atmosphere 2017, 8(11), 226; https://doi.org/10.3390/atmos8110226 - 21 Nov 2017

Cited by 21 | Viewed by 6288

Abstract

Radiocarbon analysis is a widely-used tool for source apportionment of aerosol particles. One of the big challenges of this method, addressed in this work, is to isolate elemental carbon (EC) for ¹⁴C analysis. In the first part of the study, we validate [...] Read more.

Radiocarbon analysis is a widely-used tool for source apportionment of aerosol particles. One of the big challenges of this method, addressed in this work, is to isolate elemental carbon (EC) for ¹⁴C analysis. In the first part of the study, we validate a two-step method (2stepCIO) to separate total carbon (TC) into organic carbon (OC) and EC against the EUSAAR_2 thermal-optical method regarding the recovered carbon concentrations. The 2stepCIO method is based on the combustion of OC in pure oxygen at two different temperature steps to isolate EC. It is normally used with a custom-built aerosol combustion system (ACS), but in this project, it was also implemented as a thermal protocol on a Sunset OC-EC analyzer. Results for the recovered EC mass concentration showed poor agreement between the 2stepCIO method on the ACS system and on the Sunset analyzer. This indicates that the EC recovery is sensitive not only to the temperature steps, but also to instrument-specific parameters, such as heating rates. We also found that the EUSAAR_2 protocol itself can underestimate the EC concentration on untreated samples compared to water-extracted samples. This is especially so for highly loaded filters, which are typical for ¹⁴C analysis. For untreated samples, the EC concentration on long-term filter samples (two to five days sampling time) was 20–45% lower than the sum of EC found on the corresponding 24-h filter samples. For water-extracted filter samples, there was no significant difference between long-term and the sum of daily filter samples. In the second part of this study, the ¹⁴C was measured on EC isolated by the 2stepCIO method and compared to methods from two other laboratories. The different methods agree well within their uncertainty estimates. Full article

(This article belongs to the Special Issue Carbonaceous Aerosols in Atmosphere)

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1483 KiB

Open AccessArticle

Evaluation of the MODIS C6 Aerosol Optical Depth Products over Chongqing, China

by Guangming Shi, Ruiling Liu, Ding Yi Wang and Fumo Yang

Atmosphere 2017, 8(11), 227; https://doi.org/10.3390/atmos8110227 - 20 Nov 2017

Cited by 6 | Viewed by 4143

Abstract

The Moderate Resolution Imaging Spectroradiometer (MODIS) Collection 6 (C6) aerosol optical depth (AOD) products from the 10/3 km Dark Target (DT) and Deep Blue (DB) algorithms are firstly evaluated using ground observed AODs by the sun photometer in Chongqing, a mountainous mega-city in [...] Read more.

The Moderate Resolution Imaging Spectroradiometer (MODIS) Collection 6 (C6) aerosol optical depth (AOD) products from the 10/3 km Dark Target (DT) and Deep Blue (DB) algorithms are firstly evaluated using ground observed AODs by the sun photometer in Chongqing, a mountainous mega-city in southwest China. The validation results show that MODIS AODs from 10/3 km DT algorithm are comparable with those of the sun photometer, although there are slight overestimations. However, the DB algorithm substantially underestimates MODIS AODs when comparing with those of the sun photometer. Error analyses imply that the bias of surface reflectance estimation is the main error source for both algorithms. The cloud screening scheme of the DT algorithm is more effective than the DB algorithm. The cloud vicinity effect should be considered in the quality control processes for both of the algorithms. A sensitivity test suggests that in complex terrain area, like Chongqing, the collocation method in the validation of satellite products should be carefully selected according to local circumstances. When comparing the monthly mean AODs of MODIS products with sun photometer observations, it shows that the Terra MODIS AOD products are valid to represent the mean statuses in summer and autumn, but the monthly mean of Aqua MODIS AODs are limited in Chongqing. Full article

(This article belongs to the Section Aerosols)

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3158 KiB

Open AccessArticle

Trace Metals in Cloud Water Sampled at the Puy De Dôme Station

by Angelica Bianco, Mickaël Vaïtilingom, Maxime Bridoux, Nadine Chaumerliac, Jean-Marc Pichon, Jean-Luc Piro and Laurent Deguillaume

Atmosphere 2017, 8(11), 225; https://doi.org/10.3390/atmos8110225 - 17 Nov 2017

Cited by 14 | Viewed by 4710

Abstract

Concentrations of 33 metal elements were determined by ICP-MS (Inductively Coupled Plasma Mass Spectrometry) analysis for 24 cloud water samples (corresponding to 10 cloud events) collected at the puy de Dôme station. Clouds present contrasted chemical composition with mainly marine and continental characteristics; [...] Read more.

Concentrations of 33 metal elements were determined by ICP-MS (Inductively Coupled Plasma Mass Spectrometry) analysis for 24 cloud water samples (corresponding to 10 cloud events) collected at the puy de Dôme station. Clouds present contrasted chemical composition with mainly marine and continental characteristics; for some cloud events, a further anthropogenic source can be superimposed on the background level. In this context, measurements of trace metals may help to evaluate the impact of anthropogenic and natural sources on the cloud and to better discriminate the origin of the air masses. The metal concentrations in the samples are low (between 16.4 µg L⁻¹ and 1.46 mg L⁻¹). This could be explained by the remoteness of the puy de Dôme site from local sources. Trace metals are then used to confirm and refine a previous sample classification. A principal component analysis (PCA) using the pH value and the concentrations of Cl⁻, NO₃⁻, SO₄²⁻, Na⁺ and NH₄⁺ is performed considering 24 cloud samples. This first analysis shows that 18 samples are of marine origin and 6 samples are classified as continental. The same statistical approach is used adding trace metal concentration. Zn and Mg elements are the most abundant trace metals for all clouds. A higher concentration of Cd is mainly associated to clouds from marine origins. Cu, As, Tl and Sb elements are rather found in the continental samples than in the marine ones. Mg, V, Mn and Rb elements mainly found in soil particles are also more concentrated in the samples from continental air mass. This new PCA including trace metal confirms the classification between marine and continental air masses but also indicates that one sample presenting low pH and high concentrations of SO₄²⁻, Fe, Pb and Cu could be rather attributed to a polluted event. Full article

(This article belongs to the Special Issue Atmospheric Metal Pollution)

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913 KiB

Open AccessArticle

The Summers 2003 and 2015 in South-West Germany: Heat Waves and Heat-Related Mortality in the Context of Climate Change

by Stefan Muthers, Gudrun Laschewski and Andreas Matzarakis

Atmosphere 2017, 8(11), 224; https://doi.org/10.3390/atmos8110224 - 15 Nov 2017

Cited by 93 | Viewed by 10676

Abstract

After 2003, another hot summer took place in Western and Central Europe in 2015. In this study, we compare the characteristics of the two major heat waves of these two summers and their effect on the heat related mortality. The analysis is performed [...] Read more.

After 2003, another hot summer took place in Western and Central Europe in 2015. In this study, we compare the characteristics of the two major heat waves of these two summers and their effect on the heat related mortality. The analysis is performed with focus on South-West Germany (Baden–Württemberg). With an additional mean summer mortality of +7.9% (2003) and +5.8% (2015) both years mark the top-two records of the summer mortality in the period 1968–2015. In each summer, one major heat wave contributed strongly to the excess summer mortality: In August 2003, daily mortality reached anomalies of +70% and in July 2015 maximum deviations of +56% were observed. The August 2003 heat wave was very long-lasting and characterized by exceptional high maximum and minimum temperatures. In July 2015, temperatures were slightly lower than in 2003, however, the high air humidity during the day and night, lead to comparable heat loads. Furthermore, the heat wave occurred earlier during the summer, when the population was less acclimated to heat stress. Using regional climate models we project an increasing probability for future 2003- and 2015-like heat waves already in the near future (2021–2050), with a 2015-like event occurring about every second summer. In the far future (2070–2099) pronounced increases with more than two 2015-like heat waves per summer are possible. Full article

(This article belongs to the Special Issue Impacts of Climate Change on Human Health)

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7722 KiB

Open AccessArticle

Trends and Variability in Aerosol Optical Depth over North China from MODIS C6 Aerosol Products during 2001–2016

by Peng Wang, Shangjun Ning, Jiageng Dai, Jingmin Sun, Mingjia Lv, Qingli Song, Xin Dai, Jinrong Zhao and Dajiang Yu

Atmosphere 2017, 8(11), 223; https://doi.org/10.3390/atmos8110223 - 15 Nov 2017

Cited by 22 | Viewed by 4394

Abstract

This study analyzed the variability and trend in aerosol optical depth (AOD) over North China using the latest MODIS/Terra C6 merged Dark Target/Deep Blue AOD monthly data at 550 nm from 2001 to 2016. The spatial distribution of the annual mean AOD was [...] Read more.

This study analyzed the variability and trend in aerosol optical depth (AOD) over North China using the latest MODIS/Terra C6 merged Dark Target/Deep Blue AOD monthly data at 550 nm from 2001 to 2016. The spatial distribution of the annual mean AOD was generally characterized by two prominent high-value centers located in the industrially and economically developed areas of the North China Plain and East China, and the dust aerosol-dominated areas of southern Xinjiang. The seasonally averaged AOD reached its maximum in spring (0.430 ± 0.049), followed by summer (0.356 ± 0.035) and winter (0.282 ± 0.039), with the minimum occurring in autumn (0.219 ± 0.022). There were notable long-term annual trends in AOD in different regions over North China during 2001–2016: a decreasing AOD trend was found in Qinghai Tibet (−0.015 ± 0.010/decade), Northwest China (−0.059 ± 0.013/decade at 99% confidence level), and the North China Plain (−0.007 ± 0.021/decade), but a positive increasing trend was identified in northern Xinjiang (0.01 ± 0.006/decade), southern Xinjiang (0.002 ± 0.013/decade), East China (0.053 ± 0.042/decade), and Northeast China (0.016 ± 0.029/decade). Seasonal patterns in the AOD regional long-term trend were evident. The AODs in spring over all the study regions, except East China, exhibited a decreasing trend, with the maximum trend value observed in Northwest China (−0.099 ± 0.029/decade at 99% confidence level); whereas AODs in autumn, except in Northwest China, showed an increasing trend, with the maximum trend value occurring in East China (0.073 ± 0.038/decade). Geographically, we also examined the annual and seasonal spatial patterns of AOD trends over North China. The annual spatial trends in AOD revealed a dominance of positive trends in most regions over the whole of North China from 2001 to 2016, but especially in East and Northeast China (AOD trend value of about 0.16/decade); whereas a negative trend was observed over northern Inner Mongolia (AOD trend value of about −0.12/decade). In addition, seasonal spatial trend analyses indicated that a continual clear upward trend occurred in East China in the autumn and winter seasons during the study period, with the maximum average increase occurring in winter (about 0.20/decade). Full article

(This article belongs to the Section Aerosols)

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4310 KiB

Open AccessArticle

A Quantitatively Operational Judging Method for the Process of Large Regional Heavy Haze Event Based on Satellite Remote Sensing and Numerical Simulations

by Qiao Wang, Qing Li, Zhongting Wang, Hui Chen, Huiqin Mao and Cuihong Chen

Atmosphere 2017, 8(11), 222; https://doi.org/10.3390/atmos8110222 - 15 Nov 2017

Cited by 5 | Viewed by 3950

Abstract

In recent years, large-area heavy haze pollution cases occur frequently in eastern China, especially evident in Beijing-Tianjin-Hebei and the surrounding regions. In order to operationally monitor the process of larger regional heavy haze events, a type of quantitative method based on satellite remote [...] Read more.

In recent years, large-area heavy haze pollution cases occur frequently in eastern China, especially evident in Beijing-Tianjin-Hebei and the surrounding regions. In order to operationally monitor the process of larger regional heavy haze events, a type of quantitative method based on satellite remote sensing and numerical simulations was first established and applied in multiple heavy haze processes in the research area. First, this study proposed the operational haze aerosol optical depth (HOD) method by combining Terra, Aqua satellite and WRF-NAQPM numerical simulation in haze days. Second, based on the coupled HOD data, we proposed the quantitative method for obtaining the process and severity degree for larger regional heavy haze events. Finally, this study used the method applying it to several typical heavy pollution events which occurred in Beijing-Tianjin-Hebei and its three surrounding provinces in the winter season from 1 November 2015 to 4 January 2016. The validation for HOD retrieval results showed that the couple HOD from this study have good accuracy, the linear correlation coefficient between retrieval HOD and the AERONET Beijing station data reached over 0.8, and the linear correlation coefficient between the retrieval HOD and the regional ground monitoring station PM_2.5 data reached over 0.7. The applied results showed that the method in this study is feasible to reflect the whole process of heavy haze events. Analysis of the typical heavy haze pollution events showed that the set of quantitative haze judging method in this study was consistent with the meteorological conditions in haze days also verifying that the method for haze inversion and the process analysis is reliable. Full article

(This article belongs to the Special Issue Regional Scale Air Quality Modelling)

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1024 KiB

Open AccessArticle

Contribution from Selected Organic Species to PM_2.5 Aerosol during a Summer Field Campaign at K-Puszta, Hungary

by Willy Maenhaut, Xuguang Chi, Wan Wang, Jan Cafmeyer, Farhat Yasmeen, Reinhilde Vermeylen, Katarzyna Szmigielska, Ivan A. Janssens and Magda Claeys

Atmosphere 2017, 8(11), 221; https://doi.org/10.3390/atmos8110221 - 14 Nov 2017

Cited by 10 | Viewed by 4156

Abstract

A summer field campaign was conducted at the forested background site of K-puszta in Hungary. The main aim was to assess the contribution of terpene-derived particulate organic compounds to the PM_2.5 organic carbon (OC) and of the secondary organic carbon (SOC) from [...] Read more.

A summer field campaign was conducted at the forested background site of K-puszta in Hungary. The main aim was to assess the contribution of terpene-derived particulate organic compounds to the PM_2.5 organic carbon (OC) and of the secondary organic carbon (SOC) from α-pinene to the OC. The study lasted from 24 May to 29 June 2006; the first half the weather was cold, while the second half was warm. Separate daytime and night-time PM_2.5 samples were collected with a high-volume sampler and the samples were analysed by several analytical techniques, including ion chromatography (IC) and liquid chromatography–mass spectrometry (LC/MS). The latter technique was used for measuring the terpene-derived species. Ancillary high time resolution measurements of volatile organic compounds (VOCs) were made with proton-transfer reaction–mass spectrometry. The temporal and diurnal variability of the particulate compounds and VOCs and interrelationships were examined. It was found that the monoterpenes and a number of terpene-derived particulate compounds, such as cis-pinic and cis-caric acid, exhibited a strong day/night difference during the warm period, with about 10 times higher levels during the night-time. During the warm period, the IC compounds and LC/MS compounds accounted, on average, for 3.1% and 2.0%, respectively, of the OC, whereas the contribution of SOC from α-pinene to the OC was estimated at a minimum of 7.1%. Full article

(This article belongs to the Special Issue Carbonaceous Aerosols in Atmosphere)

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1289 KiB

Open AccessArticle

Study on Extension of Standard Meteorological Data for Cities in South Korea Using ISO 15927-4

by Yeweon Kim, Hi-Kyoung Jang and Ki-Hyung Yu

Atmosphere 2017, 8(11), 220; https://doi.org/10.3390/atmos8110220 - 14 Nov 2017

Cited by 7 | Viewed by 4188

Abstract

Accurate standard meteorological data sets for each city are essential elements to assess and analyze high-performance buildings quantitatively in order to ensure that they comply with energy saving policies of the nation. ECO2, which is an assessment program of building energy in Korea, [...] Read more.

Accurate standard meteorological data sets for each city are essential elements to assess and analyze high-performance buildings quantitatively in order to ensure that they comply with energy saving policies of the nation. ECO2, which is an assessment program of building energy in Korea, has employed meteorological data of the closest city to the target location from 13 urban meteorological data references; the employment of this program has demonstrated the ability to reflect climatic differences between cities. The present study expanded urban meteorological data to ISO TRY (International Organization for Standard Test Reference Year), an international standard methodology that can calculate the data in a relatively simple manner using observed data in Korea, as much as possible in order to reflect meteorological data, including the air temperature relevant for heating and cooling energy as well as solar radiation (cooling/heating energy) for each city, that affected the assessment of building energy the most. In the present study, existing data is expanded to a show the standard meteorological data of 66 cities that can be put into the Korean assessment program (ECO2). This data considered valid meteorological data (minimum statistical period, air temperature, relative humidity, wind, and solar radiation, etc.) among manned and unmanned observational data obtained from 479 locations from 2001 to 2010. For cities other than the 66 aforementioned cities, zoning was conducted to separate cities that had and did not have the standard meteorological data using a cumulative temperature density graph. In this way, meteorological data can be available in all cities, which will enable more accurate simulation assessments on building energy. Full article

(This article belongs to the Special Issue Energy Meteorology)

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4255 KiB

Open AccessArticle

Regional Impact Assessment of Monsoon Variability on Wind Power Availability and Optimization in Asia

by Akintayo T. Abolude, Wen Zhou and Yu Ting Leung

Atmosphere 2017, 8(11), 219; https://doi.org/10.3390/atmos8110219 - 13 Nov 2017

Cited by 5 | Viewed by 4090

Abstract

Recent developments have emphasized the global impacts of climate change and have renewed commitments in renewable energy and energy meteorology. Wind energy depends largely on prevailing meteorological conditions on both local and large scales, thus, wind power optimization should aid its assessment and [...] Read more.

Recent developments have emphasized the global impacts of climate change and have renewed commitments in renewable energy and energy meteorology. Wind energy depends largely on prevailing meteorological conditions on both local and large scales, thus, wind power optimization should aid its assessment and development. This study uses ERA-Interim daily data from 1979 to 2014 to investigate the impact of the East Asian Monsoon on wind power in Asia. Wind power increase in the Bay of Bengal region as wind vectors strengthened from winter (DJF, December-January-February) to summer (JJA, June-July-August), while the predominant direction shifted to southwesterly. The influence of the South China Sea on South East Asia resulted in increased wind power that peaked in winter. Probability distribution functions for four sub-regions revealed higher probabilities of relatively lower wind speeds in JJA, except for the South East region, where most probable wind speeds were reached in winter. The capacity factor also varied by region and by season. Power generation was lowest in JJA for all the regions except the South West. The South East region also had the highest power generated over the domain. This variation of wind power impacts the amount of energy that must be supplied by non-wind sources, termed Demand Net Wind (DNW). Knowledge of DNW fluctuations thus becomes an important consideration for optimization of power plants, grid networking and reliability, and energy markets. Full article

(This article belongs to the Special Issue Energy Meteorology)

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3171 KiB

Open AccessArticle

The Multi-Wavelength Absorption Analyzer (MWAA) Model as a Tool for Source and Component Apportionment Based on Aerosol Absorption Properties: Application to Samples Collected in Different Environments

by Vera Bernardoni, Rosaria Erika Pileci, Lorenzo Caponi and Dario Massabò

Atmosphere 2017, 8(11), 218; https://doi.org/10.3390/atmos8110218 - 13 Nov 2017

Cited by 24 | Viewed by 5363

Abstract

The multi-wavelength absorption analyzer model (MWAA model) was recently proposed to provide a source (fossil fuel combustion vs. wood burning) and a component (black carbon BC vs. brown carbon BrC) apportionment of b_abs measured at different wavelengths, and to provide the BrC [...] Read more.

The multi-wavelength absorption analyzer model (MWAA model) was recently proposed to provide a source (fossil fuel combustion vs. wood burning) and a component (black carbon BC vs. brown carbon BrC) apportionment of b_abs measured at different wavelengths, and to provide the BrC Ångström Absorption exponent (α_BrC). This paper shows MWAA model performances and issues when applied to samples impacted by different sources. To this aim, the MWAA model was run on samples collected at a rural (Propata) and an urban (Milan) site in Italy during the winter period. Lower uncertainties on α_BrC and a better correlation of the BrC absorption coefficient (b_abs^BrC) with levoglucosan (tracer for wood burning) were obtained in Propata (compared to Milan). Nevertheless, the correlation previously mentioned improved, especially in Milan, when providing a priori information on α_BrC to MWAA. Possible reasons for this improvement could be the more complex mixture of sources present in Milan and the aging processes, which can affect aerosol composition, particle mixing, and size distribution. OC and EC source apportionment showed that wood burning was the dominating contributor to the carbonaceous fractions in Propata, whereas a more complex situation was detected in Milan. Simultaneous b_abs(BC) apportionment and EC measurements allowed MAC determination, which gave analogous results at the two sites. Full article

(This article belongs to the Special Issue Carbonaceous Aerosols in Atmosphere)

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Open AccessArticle

Evolution of Multispectral Aerosol Absorption Properties in a Biogenically-Influenced Urban Environment during the CARES Campaign

by Madhu Gyawali, W. Patrick Arnott, Rahul A. Zaveri, Chen Song, Bradley Flowers, Manvendra K. Dubey, Ari Setyan, Qi Zhang, Swarup China, Claudio Mazzoleni, Kyle Gorkowski, R. Subramanian and Hans Moosmüller

Atmosphere 2017, 8(11), 217; https://doi.org/10.3390/atmos8110217 - 13 Nov 2017

Cited by 10 | Viewed by 5940

Abstract

We present the evolution of multispectral optical properties through urban aerosols that have aged and interacted with biogenic emissions, resulting in stronger short wavelength absorption and the formation of moderately brown secondary organic aerosols. Ground-based aerosol measurements were made in June 2010 within [...] Read more.

We present the evolution of multispectral optical properties through urban aerosols that have aged and interacted with biogenic emissions, resulting in stronger short wavelength absorption and the formation of moderately brown secondary organic aerosols. Ground-based aerosol measurements were made in June 2010 within the Sacramento urban area (site T0) and at a 40-km downwind location (site T1) in the forested Sierra Nevada foothills area. Data on black carbon (BC) and non-refractory aerosol mass and composition were collected at both sites. In addition, photoacoustic (PA) instruments with integrating nephelometers were used to measure spectral absorption and scattering coefficients for wavelengths ranging from 355 to 870 nm. The daytime absorption Ångström exponent (AAE) indicated a modest wavelength-dependent enhancement of absorption at both sites throughout the study. From 22 to 28 June 2010, secondary organic aerosol mass increased significantly at both sites, which was due to increased biogenic emissions coupled with intense photochemical activity and air mass recirculation in the area. During this period, the median BC mass-normalized absorption cross-section (MAC) values for 405 nm and 532 nm at T1 increased by ~23% and ~35%, respectively, compared with the relatively less aged urban emissions at the T0 site. In contrast, the average MAC values for the 870 nm wavelength were similar for both sites. These results suggest the formation of moderately brown secondary organic aerosols in biogenically-influenced urban air. Full article

(This article belongs to the Special Issue Carbonaceous Aerosols in Atmosphere)

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2440 KiB

Open AccessArticle

The Air-Sea Nitrous Oxide Flux along Cruise Tracks to the Arctic Ocean and Southern Ocean

by Liyang Zhan, Man Wu, Liqi Chen, Jixia Zhang, Yuhong Li and Jian Liu

Atmosphere 2017, 8(11), 216; https://doi.org/10.3390/atmos8110216 - 13 Nov 2017

Cited by 8 | Viewed by 4516

Abstract

Nitrous oxide is a trace gas with two global environmental effects: it depletes stratospheric ozone and contributes to the greenhouse effect. Oceans are one of the most significant nitrous oxide sources; however, there are ocean areas whose contributions to the nitrous oxide budget [...] Read more.

Nitrous oxide is a trace gas with two global environmental effects: it depletes stratospheric ozone and contributes to the greenhouse effect. Oceans are one of the most significant nitrous oxide sources; however, there are ocean areas whose contributions to the nitrous oxide budget are not yet well studied. The Southern Ocean and the Arctic Ocean feature strong winds and portions that are covered by sea ice. These intense environmental conditions and the remoteness of these regions hamper fieldwork; hence, very limited data are available on the distributions and the source and sink characteristics of nitrous oxide. Using data from the 4th Chinese National Arctic Research Expedition and the 27th Chinese National Antarctic Research Expedition, the first global-scale investigation of the surface water N₂O distribution pattern, the factors influencing the N₂O distribution and the air-sea N₂O flux are discussed in this study. The results show that the tropical and subtropical regions (30° N–30° S) exhibit significant source characteristics, with a maximum air-sea flux of approximately 21.0 ± 3.9 μmol·m⁻²·d⁻¹. The high air-sea flux may result from the coastal influences and high wind speeds in certain areas. The distribution patterns of N₂O in the sub-polar regions (30° N–60° N, 30° S–60° S) transition from oversaturated to approximate equilibrium with the atmosphere, and the boundaries generally correspond with frontal structures. The distributions of N₂O in the high-latitude Southern Ocean and Arctic Ocean (>60° N and 60° S) exhibit contrasting patterns. With the exception of the continental shelf hotspot, the Arctic Ocean surface water is undersaturated with N₂O; in contrast, the high-latitude Southern Ocean along the cruise track is oversaturated with N₂O. The high-latitude Southern Ocean may act as a N₂O source, with a maximum air-sea N₂O flux of approximately 9.8 ± 0.5 μmol·m⁻²·d⁻¹ at approximately 60° S, whereas the air-sea N₂O flux of the Arctic Ocean is close to zero due to the low wind speed conditions at these latitudes. Full article

(This article belongs to the Section Biosphere/Hydrosphere/Land–Atmosphere Interactions)

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1353 KiB

Open AccessArticle

Onshore Wind Speed Modulates Microbial Aerosols along an Urban Waterfront

by M. Elias Dueker, Gregory D. O’Mullan, Joaquín Martínez Martínez, Andrew R. Juhl and Kathleen C. Weathers

Atmosphere 2017, 8(11), 215; https://doi.org/10.3390/atmos8110215 - 9 Nov 2017

Cited by 19 | Viewed by 5578

Abstract

Wind blowing over aquatic and terrestrial surfaces produces aerosols, which include microbial aerosols. We studied the effect of onshore wind speeds on aerosol concentrations as well as total and culturable microbial aerosols (bacterial and viral) at an urban waterfront (New York, NY, United [...] Read more.

Wind blowing over aquatic and terrestrial surfaces produces aerosols, which include microbial aerosols. We studied the effect of onshore wind speeds on aerosol concentrations as well as total and culturable microbial aerosols (bacterial and viral) at an urban waterfront (New York, NY, United States of America). We used two distinct methods to characterize microbial aerosol responses to wind speed: A culture-based exposure-plate method measuring viable bacterial deposition near-shore (CFU accumulation rate); and a culture-independent aerosol sampler-based method measuring total bacterial and viral aerosols (cells m⁻³ air). While ambient coarse (>2 µm) and fine (0.3–2 µm) aerosol particle number concentrations (regulated indicators of air quality) decreased with increasing onshore wind speeds, total and depositing culturable bacterial aerosols and total viral aerosols increased. Taxonomic identification of the 16S rDNA of bacterial aerosol isolates suggested both terrestrial and aquatic sources. Wind appears to increase microbial aerosol number concentrations in the near-shore environment by onshore transport at low wind speeds (<4 m s⁻¹), and increased local production and transport of new microbial aerosols from adjacent water surfaces at higher wind speeds (>4 m s⁻¹). This study demonstrates a wind-modulated microbial connection between water and air in the coastal urban environment, with implications for public health management and urban microbial ecology. Full article

(This article belongs to the Special Issue Biological Particles in Atmosphere)

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5222 KiB

Open AccessArticle

The Spatial and Temporal Variation of Temperature in the Qinghai-Xizang (Tibetan) Plateau during 1971–2015

by Zhaochen Liu, Meixue Yang, Guoning Wan and Xuejia Wang

Atmosphere 2017, 8(11), 214; https://doi.org/10.3390/atmos8110214 - 9 Nov 2017

Cited by 20 | Viewed by 4815

Abstract

The Tibetan Plateau (TP), which is well known as “The Third Pole”, is of great importance to climate change in East Asia, and even the whole world. In this paper, we selected the monthly temperature (including the monthly mean and the maximum and [...] Read more.

The Tibetan Plateau (TP), which is well known as “The Third Pole”, is of great importance to climate change in East Asia, and even the whole world. In this paper, we selected the monthly temperature (including the monthly mean and the maximum and minimum temperature) during 1971–2015 from 88 meteorological stations on the TP. The data were tested and corrected by using Penalized Maximal F Test (PMFT) based on RHtest. Afterwards, based on the Mann-Kendall test, we analyzed the seasonal and time-interval characteristics on each station in detail. The results show that the TP has experienced significant warming during 1971–2015. When comparing the selected elements, the warming rate of minimum temperature (T_min) is the largest, the mean temperature (T_mean) comes second, and the maximum temperature (T_max) is the smallest. The warming trends in four seasons are significant, and the highest warming rate occurs in winter. The warming trend on the TP has a prominent spatial difference, with a large warming rate on the eastern parts and a small one on the central regions. In different seasons, the warming trends on the TP have different characteristics in the time interval. Since 1998, the warming rate in spring increased markedly, spring has displaced winter as the season with the highest warming rate recently. Full article

(This article belongs to the Special Issue Temperature Extremes and Heat/Cold Waves)

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1029 KiB

Open AccessFeature PaperArticle

Sources and Formation Processes of Short-Chain Saturated Diacids (C₂–C₄) in Inhalable Particles (PM₁₀) from Huangshi City, Central China

by Hongxia Liu, Kimitaka Kawamura, Bhagawati Kunwar, Junji Cao, Jiaquan Zhang, Changlin Zhan, Jingru Zheng, Ruizhen Yao, Ting Liu, Xianli Liu and Wensheng Xiao

Atmosphere 2017, 8(11), 213; https://doi.org/10.3390/atmos8110213 - 8 Nov 2017

Cited by 4 | Viewed by 4153

Abstract

PM₁₀ samples were collected from Huangshi (HS) city, Central China during April 2012 to March 2013, and were analyzed for short-chain saturated dicarboxylic acids (diacids) using a capillary gas chromatograph (GC). We found that oxalic acid (C₂, 318 ± 104 [...] Read more.

PM₁₀ samples were collected from Huangshi (HS) city, Central China during April 2012 to March 2013, and were analyzed for short-chain saturated dicarboxylic acids (diacids) using a capillary gas chromatograph (GC). We found that oxalic acid (C₂, 318 ± 104 ng·m⁻³) was the most abundant diacid species, followed by malonic acid (C₃, 25.4 ± 9.11 ng·m⁻³) and succinic acid (C₄, 2.09 ± 0.52 ng·m⁻³). The concentrations of C₂ and C₄ diacids were highest in winter, followed by summer and spring, and lowest in autumn. C₃ diacid was decreased in the order of summer > winter > autumn > spring. Further, the seasonal variations of WSOC (water-soluble organic carbon)- and OC (organic carbon)-normalized diacid concentrations were similar to those of diacid concentrations, suggesting that both primary emission and secondary production are important sources for diacids in Huangshi (HS) aerosols. Strong correlations were found among C₂ diacid and the three ions SO₄²⁻, NO₃⁻, and NH₄⁺ in summer and winter, suggesting that the species could undergo a similar secondary oxidation processing. C₂ had good correlation with K⁺ in summer and autumn, which indicates an enhanced contribution of combustion sources for C₂ diacid. Moreover, according to the ratio of C₂/K⁺, we can conclude that C₂ diacid should be formed by a secondary reaction of biomass combustion in HS aerosols, especially in summer and autumn. The ratios of C₂/C₄ and C₃/C₄ were compared with those reported in other sites, and the results suggest that HS aerosols should be more photochemically aged than at other urban areas. Principal component analysis of diacids and selected water-soluble inorganic ions over four seasons suggests that HS aerosols are influenced not only from primary emission, but also from secondary reaction. According to the linear relation between C₂ and C₃ diacids, the results indicate that C₂ diacid is formed from the oxidation of hydrocarbon compounds in spring, while it is from the oxidation of C₃ and C₄ diacids in summer, autumn, and winter. Full article

(This article belongs to the Special Issue Formation and Transformation of Organic Aerosol)

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8371 KiB

Open AccessArticle

Numerical Simulations of the Impacts of Mountain on Oasis Effects in Arid Central Asia

by Miao Zhang, Geping Luo, Rafiq Hamdi, Yuan Qiu, Xinxin Wang, Philippe De Maeyer and Alishir Kurban

Atmosphere 2017, 8(11), 212; https://doi.org/10.3390/atmos8110212 - 1 Nov 2017

Cited by 10 | Viewed by 4340

Abstract

The oases in the mountain-basin systems of Central Asia are extremely fragile. Investigating oasis effects and oasis-desert interactions is important for understanding the ecological stability of oases. However, previous studies have been performed only in oasis-desert environments and have not considered the impacts [...] Read more.

The oases in the mountain-basin systems of Central Asia are extremely fragile. Investigating oasis effects and oasis-desert interactions is important for understanding the ecological stability of oases. However, previous studies have been performed only in oasis-desert environments and have not considered the impacts of mountains. In this study, oasis effects were explored in the context of mountain effects in the northern Tianshan Mountains (NTM) using the Weather Research and Forecasting (WRF) model. Four numerical simulations are performed. The def simulation uses the default terrestrial datasets provided by the WRF model. The mod simulation uses actual terrestrial datasets from satellite products. The non-oasis simulation is a scenario simulation in which oasis areas are replaced by desert conditions, while all other conditions are the same as the mod simulation. Finally, the non-mountain simulation is a scenario simulation in which the elevation values of all grids are set to a constant value of 300 m, while all other conditions are the same as in the mod simulation. The mod simulation agrees well with near-surface measurements of temperature, relative humidity and latent heat flux. The Tianshan Mountains exert a cooling and wetting effects in the NTM region. The oasis breeze circulation (OBC) between oases and the deserts is counteracted by the stronger background circulation. Thus, the self-supporting mechanism of oases originating from the OBC plays a limited role in maintaining the ecological stability of oases in this mountain-basin system. However, the mountain wind causes the “cold-wet’’ island effects of the oases to extend into the oasis-desert transition zone at night, which is beneficial for plants in the transition region. Full article

(This article belongs to the Section Biosphere/Hydrosphere/Land–Atmosphere Interactions)

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4675 KiB

Open AccessArticle

Overview of the Model and Observation Evaluation Toolkit (MONET) Version 1.0 for Evaluating Atmospheric Transport Models

by Barry Baker and Li Pan

Atmosphere 2017, 8(11), 210; https://doi.org/10.3390/atmos8110210 - 31 Oct 2017

Cited by 8 | Viewed by 7558

Abstract

This paper describes the development and initial applications of the Model and Observation Evaluation Tool (MONET) v1.0. MONET was developed to evaluate the Community Multiscale Air Quality Model (CMAQ) for the NOAA National Air Quality Forecast Capability (NAQFC) modeling system. MONET is designed [...] Read more.

This paper describes the development and initial applications of the Model and Observation Evaluation Tool (MONET) v1.0. MONET was developed to evaluate the Community Multiscale Air Quality Model (CMAQ) for the NOAA National Air Quality Forecast Capability (NAQFC) modeling system. MONET is designed to be a modularized Python package for (1) pairing model output to observational data in space and time; (2) leveraging the pandas Python package for easy searching and grouping; and (3) analyzing and visualizing data. This process introduces a convenient method for evaluating model output. MONET processes data that is easily searchable and that can be grouped using meta-data found within the observational datasets. Common statistical metrics (e.g., bias, correlation, and skill scores), plotting routines such as scatter plots, timeseries, spatial plots, and more are included in the package. MONET is well modularized and can add further observational datasets and different models. Full article

(This article belongs to the Special Issue Air Quality Monitoring and Forecasting)

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2303 KiB

Open AccessArticle

Inter-Building Effect and Its Relation with Highly Reflective Envelopes on Building Energy Use: Case Study for Cities of Japan

by Jihui Yuan, Craig Farnham and Kazuo Emura

Atmosphere 2017, 8(11), 211; https://doi.org/10.3390/atmos8110211 - 28 Oct 2017

Cited by 10 | Viewed by 4137

Abstract

The built environment with respect to building envelope designs and the surrounding micro-environment significantly affects building energy use. The influence of the inter-building effect (IBE) on building energy use cannot be ignored and thermal properties of building envelopes also largely affect building energy [...] Read more.

The built environment with respect to building envelope designs and the surrounding micro-environment significantly affects building energy use. The influence of the inter-building effect (IBE) on building energy use cannot be ignored and thermal properties of building envelopes also largely affect building energy use. In order to evaluate the influence of IBE and its relation with highly-reflective (HR) building envelopes on building energy use, the building energy use under three simulated scenarios was quantitatively analyzed using the building energy optimization software “BEopt” for five cities of Japan. Analysis indicated that when the simulated building is neighbored by other buildings, an envelope coated with HR material is more effective than lowly-reflective (LR) material to reduce building energy use. A simulated single building without surrounding buildings and a LR envelope has the highest building energy use among the three simulated scenarios. This study also showed the influence of IBE on building energy savings is stronger in cities with lower latitudes. Full article

(This article belongs to the Special Issue Recent Advances in Urban Ventilation Assessment and Flow Modelling)

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680 KiB

Open AccessPerspective

Impact of Cold Waves and Heat Waves on the Energy Production Sector

by Juan A. Añel, Manuel Fernández-González, Xavier Labandeira, Xiral López-Otero and Laura De la Torre

Atmosphere 2017, 8(11), 209; https://doi.org/10.3390/atmos8110209 - 27 Oct 2017

Cited by 92 | Viewed by 14824

Abstract

Cold and heat waves represent a significant problem for the electricity generation sector. The disruptions cold and heat waves can cause in power production are beyond their consumption impacts through, for instance, higher peak demand. Unexpected stops at thermal or nuclear power plants [...] Read more.

Cold and heat waves represent a significant problem for the electricity generation sector. The disruptions cold and heat waves can cause in power production are beyond their consumption impacts through, for instance, higher peak demand. Unexpected stops at thermal or nuclear power plants by excessively high-temperature water constitute clear examples of this. In this invited paper, we use past case studies to analyze the impact of these kinds of events on power production. Subsequently we discuss how events of this nature may evolve over the future in view of their association to climate change. Although the review is not exhaustive, we do expose some ideas that may be relevant for decision making in this area Full article

(This article belongs to the Special Issue Temperature Extremes and Heat/Cold Waves)

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19140 KiB

Open AccessArticle

Assessment of Atmospheric Wet Profiles Obtained from COSMIC Radio Occultation Observations over China

by Guirong Xu, Xinan Yue, Wengang Zhang and Xia Wan

Atmosphere 2017, 8(11), 208; https://doi.org/10.3390/atmos8110208 - 26 Oct 2017

Cited by 5 | Viewed by 4851

Abstract

Atmosperic profiles derived from Constellation Observing System for Meteorology, Ionosphere, and Climate (COSMIC) radio occultation (RO) measurements make up for the lack of operational radiosonde soundings with a high spatiotemporal distribution, and their performance over China is assessed in this paper. COSMIC-retrieved atmospheric [...] Read more.

Atmosperic profiles derived from Constellation Observing System for Meteorology, Ionosphere, and Climate (COSMIC) radio occultation (RO) measurements make up for the lack of operational radiosonde soundings with a high spatiotemporal distribution, and their performance over China is assessed in this paper. COSMIC-retrieved atmospheric wet profiles from 2014 to 2015 are compared to the contemporaneous radiosonde profiles from 120 stations, and the vertical mean differences are used. The results show that the vertical mean biases of temperature, pressure and vapor pressure are −0.10 K, 0.69 hPa and −0.01 hPa, respectively, and that for refractivity is 0.17 N. Moreover, the temperature differences are positively correlated with station altitude, yet both the pressure and vapor pressure differences are negatively correlated with station latitude, as is the refractivity difference. The large temperature difference arising from the Qinghai-Tibet Plateau (QTP) region may be associated with the complex topography of the area and the limitations in the background model used in the COSMIC profile retrieval. Furthermore, negative refractivity bias between COSMIC and radiosonde data occurs below 5 km and is large in wet southern China, with a value of less than 1%. This result may be related to more humid conditions and super-refraction. Full article

(This article belongs to the Section Meteorology)

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1750 KiB

Open AccessArticle

Observed and Projected Precipitation Changes over the Nine US Climate Regions

by Petr Chylek, Manvendra K. Dubey, Nicholas Hengartner and James D. Klett

Atmosphere 2017, 8(11), 207; https://doi.org/10.3390/atmos8110207 - 25 Oct 2017

Cited by 7 | Viewed by 6298

Abstract

We analyze the past (1900–2015) temperature and precipitation changes in nine separate US climate regions. We find that the temperature increased in a statistically significant (95% confidence level equivalent to alpha level of 0.05) manner in all of these regions. However, the variability [...] Read more.

We analyze the past (1900–2015) temperature and precipitation changes in nine separate US climate regions. We find that the temperature increased in a statistically significant (95% confidence level equivalent to alpha level of 0.05) manner in all of these regions. However, the variability in the observed precipitation was much more complex. In the eastern US (east of Rocky Mountains), the precipitation increased in all five climate regions and the increase was statistically significant in three of them. In contract, in the western US, the precipitation increased in two regions and decreased in two with no statistical significance in any region. The CMIP5 climate models (an ensemble mean) were not able to capture properly either the large precipitation differences between the eastern and the western US, or the changes of precipitation between 1900 and 2015 in eastern US. The statistical regression model explains the differences between the eastern and western US precipitation as results of different significant predictors. The anthropogenic greenhouse gases and aerosol (GHGA) are the major forcing of the precipitation in the eastern part of US, while the Pacific Decadal Oscillation (PDO) has the major influence on precipitation in the western part of the US. Our analysis suggests that the precipitation over the eastern US increased at an approximate rate of 6.7%/K, in agreement with the Clausius-Clapeyron equation, while the precipitation of the western US was approximately constant, independent of the temperature. Future precipitation over the western part of the US will depend on the behavior of the PDO, and how it (PDO) may be affected by future warming. Low hydrological sensitivity (percent increase of precipitation per one K of warming) projected by the CMIP5 models for the eastern US suggests either an underestimate of future precipitation or an overestimate of future warming. Full article

(This article belongs to the Special Issue Global Precipitation with Climate Change)

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